{"title":"A novel approach for predicting multiple key properties of water-based nanofluids using artificial neural networks","authors":"Kasim Erdem, Abdussamet Subasi","doi":"10.1016/j.molliq.2025.127590","DOIUrl":null,"url":null,"abstract":"<div><div>This study represents the first implementation of a single neural network to forecast multiple fundamental properties of water-based nanofluids rather than employing distinct neural networks for individual nanofluids and properties. For each property, 701 experimental data points for 22 different (<figure><img></figure>, <figure><img></figure>, <figure><img></figure>, ND, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure> in five different mixing ratios, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, <figure><img></figure>, and <figure><img></figure>) water-based nanofluids collected from several studies in the literature having particle volume fractions between 0.1% and 1.0% in the temperature range of 15–60<!--> <sup>∘</sup>C. In the data set, temperature, volume fraction, and type of nanoparticles are considered as inputs, while thermal conductivity, dynamic viscosity, specific heat capacity, and density are considered as outputs. The hyper-parameters of the network were determined using the Bayesian optimization approach. Additionally, the k-fold cross-validation technique has been employed to prevent overfitting and improve the performance of the network. The optimum ANN structure results were compared with empirical correlations proposed by several authors. The findings indicate that the prediction capability of ANN, having a mean square error of 1.45e-4 and a coefficient of determination of 0.997265, outperforms that of correlations, enabling the straightforward prediction of multiple key properties of the studied water-based nanofluids through a single network rather than sophisticated correlations.</div></div>","PeriodicalId":371,"journal":{"name":"Journal of Molecular Liquids","volume":"429 ","pages":"Article 127590"},"PeriodicalIF":5.3000,"publicationDate":"2025-04-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Molecular Liquids","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0167732225007573","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
This study represents the first implementation of a single neural network to forecast multiple fundamental properties of water-based nanofluids rather than employing distinct neural networks for individual nanofluids and properties. For each property, 701 experimental data points for 22 different (, , , ND, , , , , , , , , in five different mixing ratios, , , , , and ) water-based nanofluids collected from several studies in the literature having particle volume fractions between 0.1% and 1.0% in the temperature range of 15–60 ∘C. In the data set, temperature, volume fraction, and type of nanoparticles are considered as inputs, while thermal conductivity, dynamic viscosity, specific heat capacity, and density are considered as outputs. The hyper-parameters of the network were determined using the Bayesian optimization approach. Additionally, the k-fold cross-validation technique has been employed to prevent overfitting and improve the performance of the network. The optimum ANN structure results were compared with empirical correlations proposed by several authors. The findings indicate that the prediction capability of ANN, having a mean square error of 1.45e-4 and a coefficient of determination of 0.997265, outperforms that of correlations, enabling the straightforward prediction of multiple key properties of the studied water-based nanofluids through a single network rather than sophisticated correlations.
期刊介绍:
The journal includes papers in the following areas:
– Simple organic liquids and mixtures
– Ionic liquids
– Surfactant solutions (including micelles and vesicles) and liquid interfaces
– Colloidal solutions and nanoparticles
– Thermotropic and lyotropic liquid crystals
– Ferrofluids
– Water, aqueous solutions and other hydrogen-bonded liquids
– Lubricants, polymer solutions and melts
– Molten metals and salts
– Phase transitions and critical phenomena in liquids and confined fluids
– Self assembly in complex liquids.– Biomolecules in solution
The emphasis is on the molecular (or microscopic) understanding of particular liquids or liquid systems, especially concerning structure, dynamics and intermolecular forces. The experimental techniques used may include:
– Conventional spectroscopy (mid-IR and far-IR, Raman, NMR, etc.)
– Non-linear optics and time resolved spectroscopy (psec, fsec, asec, ISRS, etc.)
– Light scattering (Rayleigh, Brillouin, PCS, etc.)
– Dielectric relaxation
– X-ray and neutron scattering and diffraction.
Experimental studies, computer simulations (MD or MC) and analytical theory will be considered for publication; papers just reporting experimental results that do not contribute to the understanding of the fundamentals of molecular and ionic liquids will not be accepted. Only papers of a non-routine nature and advancing the field will be considered for publication.