Photocurrent Nanoscopy of Quantum Hall Bulk

IF 11.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY
Ran Jing, Boyi Zhou, Jiacheng Sun, Shoujing Chen, Wenjun Zheng, Zijian Zhou, Heng Wang, Lukas Wehmeier, Bing Cheng, Michael Dapolito, Yinan Dong, Zengyi Du, G. L. Carr, Xu Du, D. N. Basov, Qiang Li, Mengkun Liu
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Abstract

Understanding nanoscale electronic and thermal transport of two-dimensional (2D) electron systems in the quantum Hall regime, particularly in the bulk insulating state, poses considerable challenges. One of the primary difficulties arises from the presence of chiral edge channels, whose transport behavior obscures the investigation of the insulating bulk. Using near-field optical and photocurrent nanoscopy, we probe real-space variations of the optical and thermal dynamics of graphene in the quantum Hall regime without relying on complex sample or electrode geometries. Near the charge-neutrality point, we detect strong optical and photothermal signals from resonant inter-Landau-level (LL) magnetoexciton excitations between the zeroth and ±1 st LLs, which gradually weaken with increasing doping due to Pauli blocking. Interestingly, at higher doping levels and full-integer LL fillings, photothermal signals reappear across the entire sample over an approximately 10μm scale, indicating unexpectedly long cooling lengths and nonlocal photothermal heating through the insulating bulk. This observation suggests that thermal conductivity persists for the localized states even as electronic transport is suppressed—a clear violation of the Wiedemann-Franz law. Our experiments provide novel insights into nanoscale thermal and electronic transport in incompressible 2D gases, highlighting the roles of magnetoexcitons and chiral edge states in the thermo-optoelectric dynamics of the Dirac quantum Hall state. Published by the American Physical Society 2025
量子霍尔体的光电流纳米观察
了解量子霍尔机制下二维(2D)电子系统的纳米级电子和热传输,尤其是在体绝缘状态下的传输,是一项相当大的挑战。主要困难之一来自手性边缘通道的存在,其传输行为掩盖了对绝缘体的研究。我们利用近场光学和光电流纳米镜技术,探测了量子霍尔机制下石墨烯光学和热动力学的真实空间变化,而无需依赖复杂的样品或电极几何结构。在电荷中性点附近,我们探测到了来自第zeroth和±1st LLs之间共振的兰道级(LL)间磁激子激发的强烈光学和光热信号,由于保利阻滞,这些信号随着掺杂量的增加而逐渐减弱。有趣的是,在较高的掺杂水平和全整数 LL 填充时,光热信号会在整个样品中重新出现,范围约为 10μm,这表明通过绝缘体的冷却长度和非局部光热加热出乎意料地长。这一观察结果表明,即使电子传输被抑制,局部态的热传导性仍然存在--这明显违反了维德曼-弗兰茨定律。我们的实验为不可压缩二维气体中的纳米尺度热和电子输运提供了新的见解,突出了磁激子和手性边缘态在狄拉克量子霍尔态热-光-电动力学中的作用。 美国物理学会出版 2025
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来源期刊
Physical Review X
Physical Review X PHYSICS, MULTIDISCIPLINARY-
CiteScore
24.60
自引率
1.60%
发文量
197
审稿时长
3 months
期刊介绍: Physical Review X (PRX) stands as an exclusively online, fully open-access journal, emphasizing innovation, quality, and enduring impact in the scientific content it disseminates. Devoted to showcasing a curated selection of papers from pure, applied, and interdisciplinary physics, PRX aims to feature work with the potential to shape current and future research while leaving a lasting and profound impact in their respective fields. Encompassing the entire spectrum of physics subject areas, PRX places a special focus on groundbreaking interdisciplinary research with broad-reaching influence.
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