Comparison of greenhouse gas emission estimates from six hydropower reservoirs using modeling versus field surveys

IF 3.9 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
Rachel M. Pilla, Natalie A. Griffiths, Carly Hansen, DeMarcus Turner, Allison M. Fortner, R. Trent Jett, Michael W. Jones, Nikki J. Jones, Jana R. Phillips
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Abstract

As with most aquatic ecosystems, reservoirs play an important role in the global carbon (C) cycle and emit greenhouse gases (GHG) as carbon dioxide (CO2) and methane (CH4). However, GHG emissions from reservoirs are poorly quantified, especially in temperate systems, resulting in high uncertainty. We compared reservoir C emission estimates and uncertainty of diffusive, ebullitive, and degassing pathways in six hydropower reservoirs in the southeastern United States among four data sources: two field-based surveys and two models (including the GHG Reservoir “G-res” Tool). We found that CH4 diffusion was most similar across data sources (modeled minus observed, bias = − 21 g CO2-eq m−2 y−1) and had low relative uncertainty (coefficient of variation, CV = 0.98). On the other hand, CO2 diffusion was least consistent across data sources (bias = − 518 g CO2-eq m−2 y−1). Both field surveys indicated strong negative CO2 diffusion (i.e., CO2 uptake) at all reservoirs, while G-res estimated positive CO2 diffusion. By extension, total C emissions showed similar discrepancies, leading to high uncertainty in upscaling and interpreting reservoir source-sink dynamics. Finally, CH4 ebullition had the highest relative uncertainty (CV = 2.77) due to high variability across sites. We discuss limitations of field surveys and these models, including temperature-based annualization methods, varying definitions of ebullition zones, low sampling resolution, and lack of dynamism. Future field efforts focused on capturing variability in CO2 diffusion and CH4 ebullition will be especially valuable in reducing uncertainty and improving models to advance our understanding reservoir GHG emissions.

利用模型与实地调查对6个水电站水库温室气体排放估算的比较
与大多数水生生态系统一样,水库在全球碳(C)循环中发挥重要作用,并排放二氧化碳(CO2)和甲烷(CH4)等温室气体。然而,水库温室气体排放的量化很差,特别是在温带系统中,导致高度不确定性。我们比较了美国东南部六个水电站水库的水库C排放估算和扩散、沸腾和脱气途径的不确定性,采用了四个数据源:两个实地调查和两个模型(包括温室气体水库“G-res”工具)。我们发现CH4的扩散在不同的数据源中最为相似(模型减去观测值,偏差= - 21 g CO2-eq m - 2 y - 1),并且具有较低的相对不确定性(变异系数,CV = 0.98)。另一方面,CO2扩散在不同数据源之间最不一致(偏差= - 518 g CO2-eq m−2 y−1)。两项实地调查都表明,所有储层的CO2负扩散(即CO2吸收)都很强,而G-res估计CO2正扩散。引申而言,碳排放总量也表现出类似的差异,导致升尺度和解释储源汇动态具有很高的不确定性。最后,CH4沸腾具有最高的相对不确定性(CV = 2.77),这是由于不同地点的高变异性。我们讨论了野外调查和这些模型的局限性,包括基于温度的年化方法、不同的沸腾区定义、低采样分辨率和缺乏动态性。未来的野外工作将集中在捕获CO2扩散和CH4泡腾的变异性上,这对于减少不确定性和改进模型以推进我们对水库温室气体排放的理解将特别有价值。
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来源期刊
Biogeochemistry
Biogeochemistry 环境科学-地球科学综合
CiteScore
7.10
自引率
5.00%
发文量
112
审稿时长
3.2 months
期刊介绍: Biogeochemistry publishes original and synthetic papers dealing with biotic controls on the chemistry of the environment, or with the geochemical control of the structure and function of ecosystems. Cycles are considered, either of individual elements or of specific classes of natural or anthropogenic compounds in ecosystems. Particular emphasis is given to coupled interactions of element cycles. The journal spans from the molecular to global scales to elucidate the mechanisms driving patterns in biogeochemical cycles through space and time. Studies on both natural and artificial ecosystems are published when they contribute to a general understanding of biogeochemistry.
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