Yan Chen, Xiaoyun Wang, Sili Huang, Shiyi Song, Shanjun Chen, Jie Hou and Yan Xiong
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引用次数: 0
Abstract
Metamaterials hold great promise for application in the field of perfect absorbers due to their remarkable ability to manipulate electromagnetic waves. In this work, a full-spectrum ultra-wideband solar absorber with a multilayer metal–dielectric stacked structure is designed. Our absorber is simple and easy to manufacture, with Ti serving as the substrate, overlaid with Si3N4 spacer layers and four pairs of Ti–Si3N4 ring columns. It exhibits an average absorption rate of 98.48% from 280 to 4000 nm. The synergistic effects of cavity resonance (CR), surface plasmon resonance (SPR), and magnetic resonance (MR) effectively enhance the absorption performance. The impacts of different materials, stacked layers, and geometric parameters on the absorption performance are investigated, along with further analysis of the electromagnetic field distribution to study the physical mechanism for achieving high-efficiency absorption. Additionally, it is demonstrated that the absorber exhibits polarization-independent behavior under vertical incidence and maintains an average absorption rate of over 93% at a 50° incidence angle for transverse magnetic (TM) and transverse electric (TE) polarized light. Furthermore, the absorber achieves a total solar absorption rate of 98.07% across the entire spectrum, with a thermal radiation efficiency of over 99% and a photothermal conversion efficiency of 92.49% at 1000 K. To conclude, our absorber offers great possibilities for solar energy harvesting related applications.
期刊介绍:
Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions.
The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.