Baseline concentrations and quantitative health risk assessment of polycyclic aromatic hydrocarbons (PAHs) in relation to particle grain size in street dust of Warsaw Poland.

IF 3.2 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL
Sylwia Dytłow, Jakub Karasiński, Julio Cesar Torres-Elguera
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Abstract

Total concentrations, toxicity, and health risks of 16 polycyclic aromatic hydrocarbons (PAH) in street dust from Warsaw (Poland) in 6 granulometric fractions were investigated. Street dust was collected from 149 sampling points distributed among Area 1 (central districts, left bank of the Vistula River, mostly traffic-related pollution) and Area 2&3 (suburb area, mostly residential, right bank of the river). Street dust was investigated before ("all") and after separating into 5 size-dependent samples: (1-0.8 mm) "0.8", (0.8-0.6 mm) "0.6", (0.6-0.4 mm) "0.4", (0.4-0.2 mm) "0.2", and (below 0.2 mm) " < 0.2". ΣPAH mean concentration was 3.21 mg/kg for Area 1 and 0.89 mg/kg for Area 2&3. ∑BaPTPE values calculated collectively for Area 1&2&3 were observed to be 318.3, 83.5, 131.1, 81.4, 164.3, and 339.7 ng/g for "all", "0.6", "0.4", "0.2", and " < 0.2", respectively. Significant differences in ∑BaPTPE values were observed between fractions and specific areas. The cancer risk levels for children and adults, for all particulate size fractions, were comparable for dermal contact and by ingestion and ranged from 10-5 to 10-4, whereas the cancer risk levels via inhalation always ranged from 10-10 to 10-8. Therefore, inhalation of resuspended street dust is almost negligible compared to other pathways. Environmental implication. Street dust pollution in cities is one of the most important issues in the world and it negatively affects the quality of the environment and people's health. This study contributed to filling the gap in knowledge about the characteristics of PAH contaminants in the subject of the grain size of street dust from Poland and assessing the potential health risks. Therefore, our work has provided new significant information on PAH pollution, methods of measuring PAHs content and assessing the risk to human health, which may be useful to the scientific community, policymakers, and the general public.

波兰华沙街道尘埃中多环芳烃(PAHs)与颗粒大小相关的基线浓度和定量健康风险评估。
研究了华沙(波兰)街道灰尘中6种颗粒组分中16种多环芳烃(PAH)的总浓度、毒性和健康风险。从149个采样点收集街道粉尘,这些采样点分布在区域1(中心区,维斯瓦河左岸,主要是交通污染)和区域2和3(郊区,主要是住宅区,河右岸)。调查之前(“全部”)和之后的街道灰尘分为5个大小相关的样本:(1-0.8 mm)“0.8”,(0.8-0.6毫米)“0.6”, (0.6-0.4 mm)“0.4”, (0.4-0.2 mm)“0.2”及(小于0.2毫米)“所有”、“0.6”、“0.4”、“0.2”的区域1、2、3的TPE值分别为318.3、83.5、131.1、81.4、164.3和339.7 ng/g,“分数和特定区域之间的TPE值”。对于所有颗粒大小的部分,儿童和成人的癌症风险水平在皮肤接触和摄入方面是相当的,范围在10-5到10-4之间,而通过吸入的癌症风险水平始终在10-10到10-8之间。因此,与其他途径相比,吸入悬浮街头粉尘几乎可以忽略不计。环境暗示。城市街道粉尘污染是世界上最重要的问题之一,它对环境质量和人们的健康产生了负面影响。本研究有助于填补关于波兰街道尘埃粒径主体中多环芳烃污染物特征的知识空白,并评估其潜在的健康风险。因此,我们的工作为多环芳烃污染、多环芳烃含量的测量方法和对人类健康的风险评估提供了新的重要信息,可能对科学界、决策者和公众有用。
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来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
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