Baseline concentrations and quantitative health risk assessment of polycyclic aromatic hydrocarbons (PAHs) in relation to particle grain size in street dust of Warsaw Poland.
Sylwia Dytłow, Jakub Karasiński, Julio Cesar Torres-Elguera
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引用次数: 0
Abstract
Total concentrations, toxicity, and health risks of 16 polycyclic aromatic hydrocarbons (PAH) in street dust from Warsaw (Poland) in 6 granulometric fractions were investigated. Street dust was collected from 149 sampling points distributed among Area 1 (central districts, left bank of the Vistula River, mostly traffic-related pollution) and Area 2&3 (suburb area, mostly residential, right bank of the river). Street dust was investigated before ("all") and after separating into 5 size-dependent samples: (1-0.8 mm) "0.8", (0.8-0.6 mm) "0.6", (0.6-0.4 mm) "0.4", (0.4-0.2 mm) "0.2", and (below 0.2 mm) " < 0.2". ΣPAH mean concentration was 3.21 mg/kg for Area 1 and 0.89 mg/kg for Area 2&3. ∑BaPTPE values calculated collectively for Area 1&2&3 were observed to be 318.3, 83.5, 131.1, 81.4, 164.3, and 339.7 ng/g for "all", "0.6", "0.4", "0.2", and " < 0.2", respectively. Significant differences in ∑BaPTPE values were observed between fractions and specific areas. The cancer risk levels for children and adults, for all particulate size fractions, were comparable for dermal contact and by ingestion and ranged from 10-5 to 10-4, whereas the cancer risk levels via inhalation always ranged from 10-10 to 10-8. Therefore, inhalation of resuspended street dust is almost negligible compared to other pathways. Environmental implication. Street dust pollution in cities is one of the most important issues in the world and it negatively affects the quality of the environment and people's health. This study contributed to filling the gap in knowledge about the characteristics of PAH contaminants in the subject of the grain size of street dust from Poland and assessing the potential health risks. Therefore, our work has provided new significant information on PAH pollution, methods of measuring PAHs content and assessing the risk to human health, which may be useful to the scientific community, policymakers, and the general public.
期刊介绍:
Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people.
Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes.
The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.