Hybrid plasmonic metamaterials: towards enhanced ultra broadband and wide-angle solar absorption for energy harvesting

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL
Mahdi Rashki and Mohammad Reza Rakhshani
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引用次数: 0

Abstract

In this paper, we have investigated a hybrid metamaterial seven-layer solar absorber. The absorber has remarkable characteristics, including ultra-broadband perfect absorption capability, near-perfect absorption at wide angles, and insensitivity to polarization. The structure exhibits an average absorption of 98.05% across the spectral range of 300 to 5000 nm. Furthermore, the absorption bandwidth exceeding 90% spans more than 4950 nm. We have analyzed the absorptivity of the structure considering various optical mechanisms, including propagating surface plasmon resonance (SPR), local surface plasmon resonance (LSPR), guided-mode resonance (GMR), and magnetic resonance (MR). This solar absorber comprises two layers of SiO2–Fe and a layer of semi-oval TiN arrays. Despite specific geometric tolerances, it effectively maintains ultra-broad absorption performance from the visible to the mid-infrared (MIR) range. The structure demonstrates insensitivity to a wide range of polarization angles, up to approximately 65 degrees. This makes it a promising candidate for applications such as solar energy harvesting, thermal emitters, solar cells, and related technologies.

Abstract Image

杂化等离子体超材料:用于能量收集的增强超宽带和广角太阳能吸收
本文介绍了一种混合超材料的七层太阳能吸收体。该结构具有超宽带吸收能力、广角响应性和对极化不敏感等显著特点。吸收剂在300 ~ 5000nm光谱范围内的平均吸收率为98:05%,超过90%的吸收带宽扩展到4950nm以上。我们分析了由于各种光学原因,如传播表面等离子体共振(SPR),局部表面等离子体共振(LSPR),导模共振(GMR)和磁共振(MR)的影响,结构的吸收率。这个太阳能吸收器有两层SiO2􀀀Fe和一层TiN半椭圆形阵列。尽管有特定的几何公差,但其超宽吸收性能可以有效地保持从可见光到中红外(MIR)。该结构在宽偏振角(约65度)下表现为不敏感。这种结构可能是太阳能收集、热发射器、太阳能电池等的优秀候选材料。
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来源期刊
Physical Chemistry Chemical Physics
Physical Chemistry Chemical Physics 化学-物理:原子、分子和化学物理
CiteScore
5.50
自引率
9.10%
发文量
2675
审稿时长
2.0 months
期刊介绍: Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.
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