Signatures of the attractive interaction in spin spectra of one-dimensional cuprate chains

Zecheng Shen, Jiarui Liu, Hao-Xin Wang, Yao Wang
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Abstract

Identifying the minimal model for cuprates is crucial for explaining the high-Tc pairing mechanism. Recent photoemission experiments have suggested a significant near-neighbor attractive interaction V in cuprate chains, favoring pairing instability. To determine its strength, we systematically investigate the dynamical spin structure factors S(q,ω) using the density matrix renormalization group. Our analysis quantitatively reveals a notable softening in the two-spinon continuum, particularly evident in the intense spectrum at large momentum. This softening is primarily driven by the renormalization of the superexchange interaction, as determined by a comparison with the slave-boson theory. We also demonstrate the feasibility of detecting this spectral shift in thin-film samples using resonant inelastic x-ray scattering. Therefore, this provides a distinctive fingerprint for the attractive interaction, motivating future experiments to unveil essential ingredients in cuprates.

Abstract Image

一维铜氧化物链自旋光谱中的吸引力相互作用特征
确定铜氧化物的最小模型对于解释高锝配对机制至关重要。最近的光辐射实验表明,在铜氧化物链中存在显著的近邻吸引力相互作用 V,这有利于配对的不稳定性。为了确定其强度,我们利用密度矩阵重正化群系统地研究了动态自旋结构因子 S(q,ω)。我们的定量分析揭示了双自旋子连续体的显著软化,尤其是在大动量下的强谱中更为明显。这种软化主要是由超交换相互作用的重正化驱动的,这是由与从玻色子理论的比较确定的。我们还证明了利用共振非弹性 X 射线散射在薄膜样品中探测这种光谱偏移的可行性。因此,这为有吸引力的相互作用提供了一个独特的指纹,促使未来的实验揭示铜氧化物的基本成分。
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CiteScore
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