Can Li, Nickolay A. Krotkov, Joanna Joiner, Vitali Fioletov, Chris McLinden, Debora Griffin, Peter J. T. Leonard, Simon Carn, Colin Seftor, Alexander Vasilkov
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引用次数: 0
Abstract
Abstract. For nearly two decades, the Ozone Monitoring Instrument (OMI) aboard the NASA Aura spacecraft (launched in 2004) and the Ozone Mapping and Profiler Suite (OMPS) aboard the NASA/NOAA Suomi National Polar-orbiting Partnership (SNPP) satellite (launched in 2011) have been providing global monitoring of SO2 column densities from both anthropogenic and volcanic activities. Here, we describe the version 1 NOAA-20 (N20)/OMPS SO2 product, aimed at extending the long-term climate data record. To achieve this goal, we apply a principal component analysis (PCA) retrieval technique, also used for the OMI and SNPP/OMPS SO2 products, to N20/OMPS. For volcanic SO2 retrievals, the algorithm is identical between N20 and SNPP/OMPS and produces consistent retrievals for eruptions such as the 2018 Kilauea and 2019 Raikoke. For anthropogenic SO2 retrievals, the algorithm has been customized for N20/OMPS, considering its greater spatial resolution and reduced signal-to-noise ratio as compared with SNPP/OMPS. Over background areas, N20/OMPS SO2 slant column densities (SCD) show relatively small biases, comparable retrieval noise with SNPP/OMPS (after aggregation to the same spatial resolution), and remarkable stability with essentially no drift during 2018–2023. Over major anthropogenic source areas, the two OMPS retrievals are generally well-correlated but N20/OMPS SO2 is biased low especially for India and the Middle East, where the differences reach ~20 % on average. The reasons for these differences are not fully understood but are partly due to algorithmic differences. Better agreement (typical differences of ~10–15 %) is found over degassing volcanoes. SO2 emissions from large point sources, inferred from N20/OMPS retrievals, agree well with those based on OMI, SNPP/OMPS, and TROPOspheric Monitoring Instrument (TROPOMI), with correlation coefficients > 0.98 and overall differences < 10 %. The ratios between the estimated emissions and their uncertainties offer insights into the ability of different satellite instruments to detect and quantify SO2 sources. While TROPOMI has the highest ratios among all four sensors, ratios from N20/OMPS are slightly greater than OMI and substantially greater than SNPP/OMPS. Overall, our results suggest that the version 1 N20/OMPS SO2 product will successfully continue the long-term OMI and SNPP/OMPS SO2 data records. Efforts currently underway will further enhance the consistency of retrievals between different instruments, facilitating the development of multi-decade, coherent global SO2 datasets across multiple satellites.
Earth System Science DataGEOSCIENCES, MULTIDISCIPLINARYMETEOROLOGY-METEOROLOGY & ATMOSPHERIC SCIENCES
CiteScore
18.00
自引率
5.30%
发文量
231
审稿时长
35 weeks
期刊介绍:
Earth System Science Data (ESSD) is an international, interdisciplinary journal that publishes articles on original research data in order to promote the reuse of high-quality data in the field of Earth system sciences. The journal welcomes submissions of original data or data collections that meet the required quality standards and have the potential to contribute to the goals of the journal. It includes sections dedicated to regular-length articles, brief communications (such as updates to existing data sets), commentaries, review articles, and special issues. ESSD is abstracted and indexed in several databases, including Science Citation Index Expanded, Current Contents/PCE, Scopus, ADS, CLOCKSS, CNKI, DOAJ, EBSCO, Gale/Cengage, GoOA (CAS), and Google Scholar, among others.