Assessment of Radial Basis Function Network Method for Fractal-Like Agglomerate Dynamics

IF 1.6 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES
Chang Ma, Mingzhou Yu
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引用次数: 0

Abstract

During physical and chemical processes, aerosol particles often undergo coagulation to form Agglomerates. Agglomerates are fractal-like in a statistical sense, whose dynamical evolution of particle size distribution is governed by the population balance equation (PBE). In this study, the Radial Basis Function (RBF) method RBF is firstly extended to the solution of fractal-like agglomerate dynamics problems. The applicable conditions, and advantages and disadvantages of this method are studied. Two dynamic processes of fractal-like agglomerates, namely Brownian coagulation in the continuum regime and Brownian coagulation in the free molecular regime, are investigated. As a comparison, the sectional method (SM) is utilized as the referenced method. The initial geometric standard deviation (GSD) and the fractal dimension (\(D_{f}\)) of agglomerates are found to be the two main key factors affecting the accuracy and efficiency of the RBF. The RBF method is more suitable for calculating cases with larger GSD. As the GSD increases (i.e., GSD > 1.2), the computational efficiency and accuracy of the RBF increase accordingly. The RBF method is more suitable for calculating cases with larger \(D_{f}\). As the \(D_{f}\) decreases, the calculation error of RBF method becomes further larger, which is more obvious in the free molecular regime. Compared with the SM method, the calculation efficiency of RBF method increases by 3–4 orders of magnitude. This study provides excellent application of RBF method to the solution of the PBE.

径向基函数网络法对分形样聚集体动力学的评估
在物理和化学过程中,气溶胶粒子往往会发生凝结,形成团聚体(Agglomerates)。团聚体在统计意义上是分形的,其粒度分布的动态演化受种群平衡方程(PBE)的控制。本研究首次将径向基函数(RBF)方法 RBF 扩展到分形样团聚体动力学问题的求解中。研究了该方法的适用条件和优缺点。研究了分形样团聚体的两个动态过程,即连续体系中的布朗凝集和自由分子体系中的布朗凝集。作为比较,采用了截面法(SM)作为参照方法。研究发现,团聚体的初始几何标准偏差(GSD)和分形维数(\(D_{f}\))是影响 RBF 方法准确性和效率的两个主要关键因素。RBF 方法更适合计算 GSD 较大的情况。随着 GSD 的增大(即 GSD >1.2),RBF 的计算效率和精度也相应提高。RBF 方法更适合计算 \(D_{f}\) 较大的情况。随着 \(D_{f}\) 的减小,RBF 方法的计算误差进一步变大,这在自由分子体系中更为明显。与 SM 方法相比,RBF 方法的计算效率提高了 3-4 个数量级。本研究为 RBF 方法在 PBE 求解中的应用提供了很好的参考。
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来源期刊
Aerosol Science and Engineering
Aerosol Science and Engineering Environmental Science-Pollution
CiteScore
3.00
自引率
7.10%
发文量
42
期刊介绍: ASE is an international journal that publishes high-quality papers, communications, and discussion that advance aerosol science and engineering. Acceptable article forms include original research papers, review articles, letters, commentaries, news and views, research highlights, editorials, correspondence, and new-direction columns. ASE emphasizes the application of aerosol technology to both environmental and technical issues, and it provides a platform not only for basic research but also for industrial interests. We encourage scientists and researchers to submit papers that will advance our knowledge of aerosols and highlight new approaches for aerosol studies and new technologies for pollution control. ASE promotes cutting-edge studies of aerosol science and state-of-art instrumentation, but it is not limited to academic topics and instead aims to bridge the gap between basic science and industrial applications.  ASE accepts papers covering a broad range of aerosol-related topics, including aerosol physical and chemical properties, composition, formation, transport and deposition, numerical simulation of air pollution incidents, chemical processes in the atmosphere, aerosol control technologies and industrial applications. In addition, ASE welcomes papers involving new and advanced methods and technologies that focus on aerosol pollution, sampling and analysis, including the invention and development of instrumentation, nanoparticle formation, nano technology, indoor and outdoor air quality monitoring, air pollution control, and air pollution remediation and feasibility assessments.
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