{"title":"Influence of Homogeneous Nucleation on the Intensity of Evaporation/Condensation Processes","authors":"V. Yu. Levashov, A. P. Kryukov, I. N. Shishkova","doi":"10.1134/S1061933X23601361","DOIUrl":null,"url":null,"abstract":"<p>An approach based on the direct numerical solution of the Boltzmann kinetic equation is proposed to take into account the influence of homogeneous nucleation on the mass transfer intensity in the evaporation/condensation (recondensation) problem. On the basis of the comparison between the scales of the formation time of a critical-size droplet and the time of supersaturation propagation, it is shown that it is possible to describe the considered problem in two stages, i.e., without taking into account the influence of droplets at the first stage and with taking into account their influence at the second stage. The calculation results show that, in the case of immobile droplets, there is a strong influence of bulk condensation on the intensity of the evaporation/condensation process.</p>","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2024-04-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"92","ListUrlMain":"https://link.springer.com/article/10.1134/S1061933X23601361","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
An approach based on the direct numerical solution of the Boltzmann kinetic equation is proposed to take into account the influence of homogeneous nucleation on the mass transfer intensity in the evaporation/condensation (recondensation) problem. On the basis of the comparison between the scales of the formation time of a critical-size droplet and the time of supersaturation propagation, it is shown that it is possible to describe the considered problem in two stages, i.e., without taking into account the influence of droplets at the first stage and with taking into account their influence at the second stage. The calculation results show that, in the case of immobile droplets, there is a strong influence of bulk condensation on the intensity of the evaporation/condensation process.
期刊介绍：
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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