Effects of resonances and surface texturing on light emission in emerging thin-film devices

Pyry Kivisaari, M. Partanen, J. Oksanen
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Abstract

Recent developments in thin-film fabrication and processing open up interesting possibilities for both established and emerging optics technologies. There, one of the key questions requiring more complete understanding is by how much one can improve the performance of thin-film devices by utilizing resonance effects and surface texturation. In this work, we report on our recent theoretical investigations around two aspects of this question: (1) how much the overall (=angle and energy-integrated) emission of extremely thin ($\sim10$ nm) layers can be enhanced through cavity effects, and (2) how much resonances affect the emission of moderately thin ($>100$ nm) layers in a typical device interacting with free space (in this case an ultra-thin solar cell). Beginning with topic (1), we find that the total emission of active layers with thicknesses $<50$ nm in particular can be boosted through resonant effects by placing them in a cavity. For topic (2), the results indicate that a radiative transfer approach (i.e., one not accounting for resonant effects) can give even quantitatively accurate predictions of the total emission of moderately thin layers in a thin-film device, as long as the reflectances of the device's outer boundaries are known, and the emitting layer is not very close to optical elements supporting direct evanescent coupling (such as metal mirrors). Finally, we demonstrate that extending the self-consistent radiative transfer--drift-diffusion approach for diffusive scattering presents an interesting tool to optimize thin-film devices even with textured surfaces.
共振和表面纹理对新兴薄膜设备发光的影响
薄膜制造和加工领域的最新发展为成熟的和新兴的光学技术提供了有趣的可能性。在这方面,需要更全面了解的一个关键问题是,利用共振效应和表面纹理可以在多大程度上提高薄膜设备的性能。在这项工作中,我们报告了最近围绕这个问题的两个方面进行的理论研究:(1) 极薄($\sim10$ nm)层的整体(=角度和能量积分)发射能在多大程度上通过空腔效应得到增强;(2) 共振在多大程度上影响与自由空间相互作用的典型设备(本例中为超薄太阳能电池)中的中等厚度($>100$ nm)层的发射。从题目(1)开始,我们发现将厚度小于 50 纳米的有源层置于空腔中,可以通过共振效应提高其总发射率。对于课题(2),研究结果表明,只要知道器件外部边界的反射率,并且发射层不是非常靠近支持直接蒸发耦合的光学元件(如金属镜),辐射传递方法(即不考虑共振效应的方法)甚至可以定量准确地预测薄膜器件中中等厚度层的总发射。最后,我们证明了将自洽辐射传递--漂移扩散方法扩展到扩散散射是优化薄膜设备的有趣工具,即使是具有纹理表面的设备。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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