{"title":"Transport, dispersion, and degradation of nonpoint source contaminants during flood‐managed aquifer recharge","authors":"Zach Perzan, Kate Maher","doi":"10.1002/vzj2.20307","DOIUrl":null,"url":null,"abstract":"In water‐stressed regions of the world, the inundation of working landscapes to replenish aquifers—known as flood‐managed aquifer recharge (flood‐MAR)—has become a valuable tool for sustainable groundwater management. Due to their diverse land use histories, however, many potential recharge sites host nonpoint source contaminants (such as salts, pesticides, and fertilizers) within the vadose zone that may flush to groundwater during recharge operations. To identify the controls on contaminant migration, we perform stochastic simulations of flood‐MAR through a heterogeneous alluvial aquifer and apply transient particle tracking to evaluate conservative and reactive contaminant transport over 80 years of recharge operations. With semi‐annual recharge events, the water table begins to rise 0.13–1.84 years after the first inundation event while solutes take much longer (11 to 80 years) to transit the 45‐m thick unsaturated zone. We derive a parametric expression for the ratio of celerity (or rate of pressure transmission) to velocity of the flood‐MAR wetting front and show that this simplified expression agrees with values calculated from heterogeneous model simulations. Slow solute velocities (0.25–1.75 m year<jats:sup>−1</jats:sup>) allow for significant contaminant removal through denitrification, but the contaminant plume experiences minimal dispersion or dilution over this time, reaching the water table as a sharp front. Our results suggest that minimizing groundwater velocity and maximizing groundwater celerity during flood‐MAR should optimize increases in water supply while limiting water quality degradation.","PeriodicalId":23594,"journal":{"name":"Vadose Zone Journal","volume":"21 1","pages":""},"PeriodicalIF":2.5000,"publicationDate":"2024-02-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Vadose Zone Journal","FirstCategoryId":"89","ListUrlMain":"https://doi.org/10.1002/vzj2.20307","RegionNum":3,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
引用次数: 0
Abstract
In water‐stressed regions of the world, the inundation of working landscapes to replenish aquifers—known as flood‐managed aquifer recharge (flood‐MAR)—has become a valuable tool for sustainable groundwater management. Due to their diverse land use histories, however, many potential recharge sites host nonpoint source contaminants (such as salts, pesticides, and fertilizers) within the vadose zone that may flush to groundwater during recharge operations. To identify the controls on contaminant migration, we perform stochastic simulations of flood‐MAR through a heterogeneous alluvial aquifer and apply transient particle tracking to evaluate conservative and reactive contaminant transport over 80 years of recharge operations. With semi‐annual recharge events, the water table begins to rise 0.13–1.84 years after the first inundation event while solutes take much longer (11 to 80 years) to transit the 45‐m thick unsaturated zone. We derive a parametric expression for the ratio of celerity (or rate of pressure transmission) to velocity of the flood‐MAR wetting front and show that this simplified expression agrees with values calculated from heterogeneous model simulations. Slow solute velocities (0.25–1.75 m year−1) allow for significant contaminant removal through denitrification, but the contaminant plume experiences minimal dispersion or dilution over this time, reaching the water table as a sharp front. Our results suggest that minimizing groundwater velocity and maximizing groundwater celerity during flood‐MAR should optimize increases in water supply while limiting water quality degradation.
期刊介绍:
Vadose Zone Journal is a unique publication outlet for interdisciplinary research and assessment of the vadose zone, the portion of the Critical Zone that comprises the Earth’s critical living surface down to groundwater. It is a peer-reviewed, international journal publishing reviews, original research, and special sections across a wide range of disciplines. Vadose Zone Journal reports fundamental and applied research from disciplinary and multidisciplinary investigations, including assessment and policy analyses, of the mostly unsaturated zone between the soil surface and the groundwater table. The goal is to disseminate information to facilitate science-based decision-making and sustainable management of the vadose zone. Examples of topic areas suitable for VZJ are variably saturated fluid flow, heat and solute transport in granular and fractured media, flow processes in the capillary fringe at or near the water table, water table management, regional and global climate change impacts on the vadose zone, carbon sequestration, design and performance of waste disposal facilities, long-term stewardship of contaminated sites in the vadose zone, biogeochemical transformation processes, microbial processes in shallow and deep formations, bioremediation, and the fate and transport of radionuclides, inorganic and organic chemicals, colloids, viruses, and microorganisms. Articles in VZJ also address yet-to-be-resolved issues, such as how to quantify heterogeneity of subsurface processes and properties, and how to couple physical, chemical, and biological processes across a range of spatial scales from the molecular to the global.