Comparative analytical and numerical investigation of the plasma density in atmospheric air generated by nanosecond laser pulses

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
H Delibašić Marković, K Kaleris, N A Papadogiannis, V Petrović
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引用次数: 0

Abstract

Energy deposition via laser-induced breakdown (LIB) in gases or other media and its accompanying secondary light and sound radiative processes are nowadays increasingly deployed in scientific and technological applications. The modeling and control of the breakdown and radiative processes occurring by the interactions of the free electrons with the heavy particles in the partially ionized medium, requires precise spatio-temporal description of the generated free electron density. This work presents an analysis of a free electron rate model describing the free electron density in air plasmas produced by nanosecond laser pulses. The model accounts for multiphoton and cascade ionization, and for electron diffusion, recombination, and attachment. A closed-form expression of the rate model is derived and validated by comparison with experimentally validated numerical solutions, showing very good agreement in a wide range of parameters. Simulation results are presented for different laser pulses and focal spot sizes and analysis is carried out regarding the dependence of the air plasma on the various laser radiation parameters. The presented approach is particularly useful for complex multi-scale models calculating the electron and ion temperature evolution, the thermoelastic expansion and the shock-wave following LIB of gases.
纳秒激光脉冲在大气中产生的等离子体密度的分析和数值比较研究
如今,通过激光诱导击穿(LIB)在气体或其他介质中进行能量沉积及其伴随的二次光和声音辐射过程在科学和技术应用中的应用日益广泛。要对自由电子与部分电离介质中的重粒子相互作用产生的击穿和辐射过程进行建模和控制,需要对产生的自由电子密度进行精确的时空描述。这项研究对自由电子速率模型进行了分析,该模型描述了纳秒激光脉冲产生的空气等离子体中的自由电子密度。该模型考虑了多光子和级联电离,以及电子扩散、重组和附着。得出了速率模型的闭式表达式,并通过与实验验证的数值解进行比较进行了验证,结果表明在很大的参数范围内两者的一致性非常好。仿真结果显示了不同激光脉冲和焦斑大小的情况,并分析了空气等离子体对各种激光辐射参数的依赖性。该方法特别适用于计算电子和离子温度演变、热弹性膨胀和冲击波跟随气体 LIB 的复杂多尺度模型。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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