Xingyu Chen, Mengqi Li, Quanzhi Zhang, Tao Peng, Z. Xiong
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引用次数: 0
Abstract
The discharge morphology of pulsed dielectric barrier discharge (PDBD) plays important roles in its applications. Here, we systematically investigated the effects of voltage amplitude, discharge gap, and O2 content on the PDBD morphology, and revealed the possible underlying mechanism of the U-shape formation. First, the morphological evolution under different conditions were recorded. A unique U-shape region appears in the middle edge region when the gap is larger than 2 mm, while the entire discharge region remains columnar under a 2 mm gap in He PDBD. The width of the discharge and the U-shape region increase with the increase of voltage and decreases with the increase of the gap and O2 content. To explain this phenomenon, then a two-dimensional symmetric model was developed to simulate the spatiotemporal evolution of different species and calculate the electric thrust. The discharge morphology evolution directly corresponds to the excited state atomic reduction process. The electric thrust on the charged particles mainly determines the reaction region and strongly influences the U-shape formation. When the gap is less than 2 mm, the electric thrust is homogeneous throughout the entire region, resulting in a columnar shape. However, when the gap is larger than 2 mm or O2 is added, the electric thrust in the edge region becomes greater than that in the middle, leading to the U-shape formation. Furthermore, in He PDBD, the charged particles generating electric thrust are mainly electrons and helium ions, while in He/O2 PDBD those generate electric thrust at the outer edge of the electrode surface are mainly various oxygen-containing ions.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.