The Role of Diffusive Mixing in Current and Future Aviation Fuels at Relevant Operating Conditions

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Francesco Di Sabatino, Kevin Wan, Julien Manin, Tyler Capil, Yolanda Hicks, Alex Gander, Cyril Crua
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Abstract

Abstract With aviation's dependence on the high volumetric energy density offered by liquid fuels, Sustainable Aviation Fuels (SAFs) could offer the fastest path towards the decarbonization of aircrafts. However, the chemical properties of SAFs present new challenges, and research is needed to better understand their injection, combustion and emission processes. One of these processes in particular is about droplet evaporation at relevant pressures and temperatures, and this represents the focus of the present manuscript. To address this gap we characterized the evaporation and mixing of spray droplets at conditions relevant to modern and next generation aero-engine combustors. We tested three fuels from the National Jet Fuel Combustion Program, namely an average Jet A fuel (A-2), an alcohol-to-jet fuel (C-1), and a blend made of 40 % C-1 and 60 % iso-paraffins (C-4). We also tested a single component normal alkane: n-dodecane, as well as an advanced bio-derived cyclo-alkane fuel: bicyclohexyl. The time evolution of fuel droplets was monitored using high-speed long-distance microscopy. The collected images were processed using a purposely-developed and trained machine learning (ML) algorithm to detect and characterize the droplets' evaporation regime. The results revealed different evaporation regimes, such as classical and diffusive. In agreement with previous studies, evaporation regimes appear to be controlled by ambient pressure, temperature, and fuel type. The measurements demonstrate that diffusive evaporation is relevant at high-pressure conditions, such as take-off combustor pressures for modern commercial aircraft engines.
在相关操作条件下,扩散混合在当前和未来航空燃料中的作用
随着航空对液体燃料所提供的高体积能量密度的依赖,可持续航空燃料(SAFs)可以为飞机脱碳提供最快的途径。然而,saf的化学性质提出了新的挑战,需要更好地研究其喷射、燃烧和排放过程。其中一个特别的过程是关于液滴蒸发在相关的压力和温度,这代表了目前的手稿的重点。为了解决这一差距,我们在与现代和下一代航空发动机燃烧室相关的条件下表征了喷雾液滴的蒸发和混合。我们测试了三种来自国家航空燃料燃烧计划的燃料,即一种普通的航空燃料(A-2),一种酒精制航空燃料(C-1),以及一种由40%的C-1和60%的异石蜡(C-4)组成的混合物。我们还测试了一种单组分正常烷烃:正十二烷,以及一种先进的生物衍生环烷烃燃料:双环己基。利用高速远距显微镜对燃料液滴的时间演化进行了监测。收集的图像使用专门开发和训练的机器学习(ML)算法进行处理,以检测和表征液滴的蒸发状态。结果显示了不同的蒸发方式,如经典蒸发和扩散蒸发。与先前的研究一致,蒸发机制似乎受环境压力、温度和燃料类型的控制。测量结果表明,扩散蒸发与高压条件有关,例如现代商用飞机发动机的起飞燃烧室压力。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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