Diffusion limited aggregation, resetting and large deviations of Brownian motion

IF 1.6 4区 化学 Q4 CHEMISTRY, PHYSICAL
Uriel Villanueva-Alcalá, José R. Nicolás-Carlock, Denis Boyer
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引用次数: 1

Abstract

AbstractModels of fractal growth commonly consider particles diffusing in a medium and that stick irreversibly to the forming aggregate when making contact for the first time. As shown by the well-known diffusion limited aggregation (DLA) model and its generalisations, the fractal dimension is sensitive to the nature of the stochastic motion of the particles. Here, we study the structures formed by finite-lived Brownian particles, i.e. particles constrained to find the aggregate within a prescribed time, and which are removed otherwise. This motion can be modelled by diffusion with stochastic resetting, a class of processes which has been widely studied in recent years. In the short lifetime limit, a very small fraction of the particles manage to reach the aggregate. Hence, growth is controlled by atypical Brownian trajectories, that move nearly in straight line according to a large deviation principle. In d dimensions, the resulting fractal dimension of the aggregate decreases from the DLA value and tends to 1, instead of increasing to d as expected from ballistic aggregation. In the zero lifetime limit one recovers the non-trivial model of ‘aggregation by the tips’ proposed long ago by R. Jullien [J. Phys. A: Math. Gen. 19, 2129 (1986)].KEYWORDS: Brownian motionresetting processesdiffusion limited aggregationlarge deviationsgeometrical optics Disclosure statementNo potential conflict of interest was reported by the author(s).Additional informationFundingWe thank Carlos E. López Natarén for technical computer support. We acknowledge support from Consejo Nacional de Ciencia y Tecnología (Ciencia de Frontera 2019 (CONACYT)) [grant number 263958].
扩散限制聚集、重置和布朗运动的大偏差
分形生长模型通常考虑颗粒在介质中扩散,并且在第一次接触时不可逆地粘在形成的聚集体上。众所周知的扩散有限聚集(DLA)模型及其推广表明,分形维数对粒子随机运动的性质很敏感。在这里,我们研究了由有限寿命布朗粒子形成的结构,即在规定时间内找到聚集体的粒子,否则就会被移除。这种运动可以用带有随机重置的扩散来模拟,这是近年来被广泛研究的一类过程。在较短的寿命极限内,只有极小部分的颗粒能够到达聚集体。因此,增长是由非典型布朗轨迹控制的,这种轨迹根据大偏差原理几乎是直线运动的。在d维中,聚合体的分形维数从DLA值开始下降,并趋于1,而不是像弹道聚集所期望的那样增加到d。在零寿命极限下,人们恢复了R. Jullien很久以前提出的“尖端聚合”的非平凡模型[J]。理论物理。答:数学。创19,2129(1986)]。关键词:布朗运动重置过程扩散有限聚集大偏差几何光学披露声明作者未报告潜在的利益冲突。我们感谢Carlos E. López natar文职人员提供的计算机技术支持。我们感谢国家科学委员会通过Tecnología(科学前沿2019 (CONACYT))[批准号263958]的支持。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Molecular Physics
Molecular Physics 物理-物理:原子、分子和化学物理
CiteScore
3.60
自引率
5.90%
发文量
269
审稿时长
2 months
期刊介绍: Molecular Physics is a well-established international journal publishing original high quality papers in chemical physics and physical chemistry. The journal covers all experimental and theoretical aspects of molecular science, from electronic structure, molecular dynamics, spectroscopy and reaction kinetics to condensed matter, surface science, and statistical mechanics of simple and complex fluids. Contributions include full papers, preliminary communications, research notes and invited topical review articles.
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