Ultra-low radioactivity flexible printed cables

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Isaac J. Arnquist, Maria Laura di Vacri, Nicole Rocco, Richard Saldanha, Tyler Schlieder, Raj Patel, Jay Patil, Mario Perez, Harshad Uka
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引用次数: 2

Abstract

Abstract Flexible printed cables and circuitry based on copper-polyimide materials are widely used in experiments looking for rare events due to their unique electrical and mechanical characteristics. However, past studies have found copper-polyimide flexible cables to contain 400-4700 pg 238 U/g, 16-3700 pg 232 Th/g, and 170-2100 ng nat K/g, which can be a significant source of radioactive background for many current and next-generation ultralow background detectors. This study presents a comprehensive investigation into the fabrication process of copper-polyimide flexible cables and the development of custom low radioactivity cables for use in rare-event physics applications. A methodical step-by-step approach was developed and informed by ultrasensitive assay to determine the radiopurity in the starting materials and identify the contaminating production steps in the cable fabrication process. Radiopure material alternatives were identified, and cleaner production processes and treatments were developed to significantly reduce the imparted contamination. Through the newly developed radiopure fabrication process, fully-functioning cables were produced with radiocontaminant concentrations of 20-31 pg 238 U/g, 12-13 pg 232 Th/g, and 40-550 ng nat K/g, which is significantly cleaner than cables from previous work and sufficiently radiopure for current and next-generation detectors. This approach, employing witness samples to investigate each step of the fabrication process, can hopefully serve as a template for investigating radiocontaminants in other material production processes.
超低放射性柔性印刷电缆
摘要基于铜聚酰亚胺材料的柔性印刷电缆和电路由于其独特的电气和机械特性而广泛应用于寻找罕见事件的实验中。然而,过去的研究发现,铜聚酰亚胺柔性电缆含有400-4700 pg 238 U/g, 16-3700 pg 232 Th/g和170-2100 ng nat K/g,这可能是许多当前和下一代超低背景探测器的重要放射性背景来源。本研究对铜聚酰亚胺柔性电缆的制造工艺和用于罕见事件物理应用的定制低放射性电缆的开发进行了全面的研究。一种有条不紊的一步一步的方法被开发出来,并通过超灵敏分析来确定起始材料中的放射性纯度,并确定电缆制造过程中的污染生产步骤。确定了放射性材料替代品,并开发了更清洁的生产工艺和处理方法,以显著减少所带来的污染。通过新开发的放射线制作工艺,可以生产出功能齐全的电缆,其放射性污染物浓度为20-31 pg 238 U/g, 12-13 pg 232 Th/g, 40-550 ng nat K/g,比以前的电缆清洁得多,并且可以为当前和下一代探测器提供足够的放射线。这种方法采用见证样品来研究制造过程的每一步,有望作为研究其他材料生产过程中放射性污染物的模板。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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