Analytical model for luminescence enhancement by metal nanoparticles

G. Sun, J. Khurgin
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Abstract

We report a simple yet rigorous analytical model that adequately describes the luminescence enhancement of optical emitters that are placed in the vicinity of metal nanoparticles of sub-wavelength dimensions. Using the example of Au nanospheres embedded in the GaN dielectric, we show that enhancement depends strongly on the original radiative efficiency of the emitter, the nanoparticle size, and the separation between the emitter and metal nanosphere. We demonstrate that strong enhancement favors the closely spaced emitters and metal nanospheres, but putting them too close to each other does not always produce additional enhancement. Thus our model provides analytical treatment of the luminescence quenching and can be used to optimize both nanoparticle size and its separation from the emitter to yield maximum enhancement factor.
金属纳米颗粒增强发光的分析模型
我们报告了一个简单而严谨的分析模型,该模型充分描述了放置在亚波长尺寸的金属纳米颗粒附近的光发射器的发光增强。以金纳米球嵌入氮化镓电介质为例,我们发现增强与发射极的原始辐射效率、纳米颗粒的大小以及发射极与金属纳米球之间的距离密切相关。我们证明了强增强有利于紧密间隔的发射体和金属纳米球,但将它们彼此放置得太近并不总是产生额外的增强。因此,我们的模型提供了发光猝灭的分析处理,并可用于优化纳米颗粒的尺寸及其与发射器的分离,以产生最大的增强因子。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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