Study of the Cross-Section for the 122Te(γ, n)121Te Reaction by the Activation Method

O. Pop, V. Mazur, P. Derechkei, Z. Bigan
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引用次数: 1

Abstract

Relevance. The study of photonuclear reactions plays a defining role in the formation of modern ideas about highlocalized collective excitations in nuclei of the giant resonance type. The giant dipole E1-resonance (GR) is the main feature in γ-quantum absorption cross-sections of nuclei. The presence of isotopes with multiple isotopes makes it possible to trace the evolution of GR characteristics from changes in the number of neutrons in the nuclei. One such element is tellurium. Purpose. The purpose of this research is an experimental and theoretical study of the cross-section of 122Te(γ, n)121Te reaction in the region of giant E1-resonance energies. Methods. The study of the cross-section of (γ, n) reaction on 122Te isotope was performed on the bremsstrahlung γ-beam of the M-30 microtron of the Institute of Electronic Physics of the National Academy of Sciences of Ukraine. The yield curves were measured in the range of maximum gamma-quantum energies Eγmax=10-18 MeV. The reaction cross-section was calculated by the inverse matrix method. When registering the reaction products, an activation technique was used, while the gamma activity of the products was recorded by the spectrometric method. The theoretical calculations of the cross-section for the 122Te(γ, n)121Te reaction were performed using the TALYS-1.9 software package. Results. The measured experimental yield ratios of the 122Te(γ, n)121Te і 130Te(γ, n)129Te d= Yn121 /Yn129 = f (E max) reactions allowed the experimental cross-section for the 122Te(γ, n)121Te reaction to be calculated. The cross-section has a single hump shape with a maximum at an energy of ~ 15.3 MeV. It was approximated by the Lorentz curve with the parameters δ0 =(274.1±2.1) MB, Е0 (15.27±0.10) MeV, Г0 =(4.76±0.08) MeV. The cross-section obtained was compared with similar cross-sections for 126Te and 130Te isotopes, as well as with theoretical calculations according to the TALYS-1.9 program. Conclusions. The obtained cross-section for the 122Te(γ, n)121Te reaction is consistent with the evolution of the parameters of (γ, n) reaction cross-section on tellurium isotopes 130Te(γ, n)129Te with a change in the number of neutrons. The theoretical approaches used are satisfactorily consistent with the experimental data. This agreement indicates the main contribution of the statistical mechanism to the cross-section of the considered (γ, n) reaction and a relatively small contribution of semi-direct processes
活化法研究122Te(γ, n)121Te反应的截面
的相关性。光核反应的研究在巨共振型核的高局域集体激发的现代观念的形成中起着决定性的作用。巨偶极子e1共振(GR)是原子核γ-量子吸收截面的主要特征。多同位素的存在使得从核中中子数的变化来追踪GR特征的演化成为可能。其中一种元素就是碲。本研究的目的是对122Te(γ, n)121Te反应在巨e1共振能量区域的截面进行实验和理论研究。在乌克兰国家科学院电子物理研究所的M-30微管轫致γ束流上对122Te同位素(γ, n)反应的截面进行了研究。在最大γ -量子能e - γmax=10-18 MeV范围内测量了产率曲线。用逆矩阵法计算了反应截面。在记录反应产物时,使用了活化技术,而产物的伽马活度是用光谱法记录的。采用TALYS-1.9软件包对122Te(γ, n)121Te反应截面进行理论计算。通过测量122Te(γ, n)121Te与130Te(γ, n)129Te反应的实验产率比,可以计算出122Te(γ, n)121Te反应的实验截面。截面呈单一驼峰形状,最大能量为~ 15.3 MeV。用Lorentz曲线表示,δ0 =(274.1±2.1)MB, Е0(15.27±0.10)MeV, Г0 =(4.76±0.08)MeV。得到的截面与126Te和130Te同位素的相似截面进行了比较,并与根据TALYS-1.9程序进行的理论计算进行了比较。得到的122Te(γ, n)121Te反应截面与碲同位素130Te(γ, n)129Te (γ, n)反应截面参数随中子数变化的演化一致。所采用的理论方法与实验数据吻合得很好。这种一致性表明统计机制对所考虑的(γ, n)反应截面的主要贡献和半直接过程的相对较小的贡献
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