Study on the Enhancement of Diamond Fluorescence Characteristics by Multi-layer Anti-reflection Coating

Xuejiao Li, Libo Zhao, Zhikang Li, Guoxi Luo, Mingzhi Yu, Yintao Ma, Lei Li, Xudong Fang, Zhuangde Jiang
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Abstract

Quantum sensing has become a rapidly growing research within the area of sensor, which can break through the limits of traditional physical sensing and make sensing accuracy to the nanometer scale. Meanwhile nitrogen-vacancy (NV) center in bulk diamond as a sensor has varieties of applications because of its excellent characteristics. However, there are large optical reflection and low fluorescence collection efficiency at the diamond-air interface because of the large refractive index gap between diamond and air, thereby reducing the sensing sensitivity. In this work, we report a multi-layer anti-reflection coating and fabrication on the surface of diamond with genetic algorithm to solve optimization value of the average reflectance $R_{ave}$ in the wavelength range of 600–800 nm. And we fabricate SiO2-Si3N4 double-layer anti-reflection coating on diamond substrate by plasma chemical vapor deposition. Experiment results show that with an anti-reflection coating, the fluorescence collection efficiency is significantly improved, and the average transmittance in the wavelength range of 600–800 nm is increased from 82.8% to 96.7%.
多层增透涂层增强金刚石荧光特性的研究
量子传感技术突破了传统物理传感技术的局限,使传感精度达到纳米级,是传感器领域中一个快速发展的研究方向。同时,金刚石中氮空位(NV)中心由于其优异的特性而具有多种用途。然而,由于金刚石与空气之间的折射率间隙较大,在金刚石-空气界面处存在较大的光学反射和较低的荧光收集效率,从而降低了传感灵敏度。本文采用遗传算法在金刚石表面制备多层增透涂层,求解600 ~ 800 nm波长范围内平均反射率$R_{ave}$的最优值。采用等离子体化学气相沉积的方法在金刚石基体上制备了SiO2-Si3N4双层增透涂层。实验结果表明,增透涂层显著提高了荧光收集效率,在600 ~ 800 nm波长范围内的平均透过率由82.8%提高到96.7%。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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