Transport and concentration of uranium isotopes in the Laguna del Cuervo, Chihuahua, Mexico

Victoria Pérez-Reyes, R. M. Cabral-Lares, C. Méndez-García, C. Caraveo-Castro, I. Reyes-Cortés, Jorge Carrillo-Flores, M. E. Montero-Cabrera
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Abstract

In Chihuahua, an important source of environmental radioactivity is found in the Sierra Peña Blanca, in the center of the state. The site comprises about 70% of uranium reserves in Mexico. The uranium of Peña Blanca was explored and partially exploited in the '80s. Due to the closure of operations, the extracted and unprocessed ore (hundreds of tons) was confined to rocky stacks, exposed to weathering. Subject to leaching, this uranium is transported from the mountains to Laguna del Cuervo. The mineral exposed in the repository and the uranium transport by surface water and recent sediments must be studied, to assess the effects on the environment, with radiometric and materials science techniques in conventional laboratories and synchrotron light. This work presents the study of sediment and pore water samples at various points along the lagoon, and the values of the activity ratio of the 234U/238U isotopes and the sediment-water distribution coefficient of these isotopes, obtained by applying uranium liquid scintillation alpha spectrometry, gamma-ray spectrometry, scanning electron microscopy and X-ray diffraction methods.
墨西哥奇瓦瓦州库尔沃湖铀同位素的迁移和浓度
在奇瓦瓦州,一个重要的环境放射性源位于该州中心的Peña布兰卡山脉。这里的铀储量约占墨西哥铀储量的70%。Peña Blanca的铀在80年代被勘探和部分开采。由于关闭作业,开采和未加工的矿石(数百吨)被限制在岩石堆中,暴露在风化下。经过浸出,这些铀会从山上运到库尔沃湖。必须利用传统实验室和同步加速器的辐射测量和材料科学技术,研究贮存库中暴露的矿物以及地表水和近期沉积物对铀的输送,以评估对环境的影响。本文采用铀液闪烁α光谱法、伽马射线能谱法、扫描电镜法和x射线衍射法,对环礁湖不同地点的沉积物和孔隙水样品进行了研究,得到了234U/238U同位素的活度比值和沉积物-水分布系数。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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