Surface enhanced Raman scattering and photo-luminescence through Bloch surface waves in dielectric multilayers

S. Pirotta, X. Xu, A. Delfan, S. Mysore, S. Maiti, G. Dacarro, M. Patrini, G. Guizzetti, D. Bajoni, J. Sipe, G. Walker, M. Liscidini, M. Galli
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Abstract

In this work we study the Surface Enhanced Raman Scattering (SERS) via Bloch Surface Waves (BSWs) in a dielectric multi-layered structure. When the pump beam is resonantly coupled to the BSW, our results demonstrate a lower bound for the SERS-enhancement of about 50. A photo-luminescence (PL) experiment performed on the same structure shows an emission enhancement in excess of two orders of magnitude, suggesting an actual SERS-enhancement of 200, in agreement with theoretical calculations. These findings suggest that purely dielectric BSW-based structures can be a valid alternative to plasmonic substrates for enhanced Raman and photo-luminescence spectroscopy.
介质多层膜中布洛赫表面波的表面增强拉曼散射和光致发光
本文研究了介质多层结构中布洛赫表面波对表面增强拉曼散射(SERS)的影响。当泵浦光束与BSW共振耦合时,我们的结果表明sers增强的下界约为50。在同一结构上进行的光致发光(PL)实验表明,发射增强超过两个数量级,表明实际的sers增强为200,与理论计算一致。这些发现表明,纯介电bsw结构可以作为等离子体衬底的有效替代品,用于增强拉曼光谱和光致发光光谱。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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