Photonic and phononic properties of the photoluminescent diamond lattice before and after implantation (Conference Presentation)

S. N. Shibu, Dzianis Saladukha, K. An, T. Ochalski
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Abstract

This study is focused on the properties of the diamond lattice before and after implantation. The diamond lattices with nitrogen-vacancy centres have very exciting properties and they can be used in a plethora of applications from quantum sensing to biomarkers. Characteristic transmission, scattering and photoluminescence of diamond lattice with nitrogen-vacancy centres (NV-) were studied through different techniques at different temperatures. The luminescence of the synthesised diamonds was studied at a 532nm excitation wavelength and recorded in the range of 500-1100nm. Since its intensity decreases with decreasing the number of nitrogen-vacancy centres. Also, we analysed the luminescence depend on the functional groups attached to the diamond surface. Raman spectroscopy studies provide interesting results about the phonon confinement effect, structure composition and homogeneity of the material and information about the functional groups attached above the diamond surface. Raman spectra depend on the structure, purity, sp3/sp2 ratio, crystal size and surface chemistry. With increasing sp3 carbon content the intensity of the diamond peak increases, while the D-band in the Raman spectra weakens. Also, we analysed the shifts in the energy and linewidth of the diamond peak in the Raman spectra. The recent development of novel super-resolution imaging techniques coincides with the efforts to synthesize optically bright and stable biomarkers. In the future, we can use the differently doped nanodiamond fluorophores as biomarkers for sensing and bioimaging.
光致发光金刚石晶格植入前后的光子和声子性质(会议报告)
本文主要研究了植入前后金刚石晶格的性质。具有氮空位中心的金刚石晶格具有非常令人兴奋的性质,它们可以用于从量子传感到生物标志物的大量应用。采用不同的技术研究了氮空位中心(NV-)金刚石晶格在不同温度下的透射、散射和光致发光特性。在532nm激发波长下对合成金刚石的发光进行了研究,并在500-1100nm范围内进行了记录。由于其强度随氮空位中心数目的减少而减小。此外,我们还分析了金刚石表面官能团的发光特性。拉曼光谱研究提供了关于声子约束效应、材料的结构组成和均匀性以及附着在金刚石表面上的官能团的信息的有趣结果。拉曼光谱取决于结构、纯度、sp3/sp2比、晶体尺寸和表面化学。随着sp3碳含量的增加,金刚石峰的强度增加,而拉曼光谱中的d波段减弱。此外,我们还分析了喇曼光谱中金刚石峰的能量和线宽的变化。近年来,新型超分辨率成像技术的发展与合成光学明亮和稳定的生物标志物的努力相一致。在未来,我们可以使用不同掺杂的纳米金刚石荧光团作为传感和生物成像的生物标志物。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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