Dynamic Proton Gating via Interfacial Water Programming Enables Near-Unity CO2-to-CO Conversion in Acid

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DOI:10.1021/acscatal.6c01416
作者：Shen Cheng,?, ,?Xupeng Qin,?, ,?Mengting Li,?, ,?Chengrang Leng,?, ,?Haixin Sun,?, ,?Qizheng An,?, ,?Rui Li,?, ,?Jingqiu Shang,?, ,?Yaling Jiang,?, ,?Yuanli Li*,?, ,?Xin Chen*,?, ,?Mikhail Soldatov,?,
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Abstract：The efficient electroreduction of CO2 in acidic electrolytes is severely limited by the dominant hydrogen evolution reaction (HER). This challenge is exacerbated at hydrophobic interfaces, w

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