冷BaRb+分子在Rb原子超冷云中的生与死

Amir Mohammadi, A. Krükow, A. Mahdian, M. Deiss, J. Pérez-Ríos, H. da Silva, M. Raoult, O. Dulieu, J. Hecker Denschlag
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引用次数: 23

摘要

我们研究了单个BaRb$^+$分子与超冷Rb原子连续碰撞时的演化过程。最初的弱结合分子可以经历一系列弹性、非弹性、反应性和辐射性过程。我们通过开发区分不同离子种类、电子态和离子动能范围的方法来研究这些过程。通过将测量结果与模型计算结果进行比较,我们获得了离子通过多种可用的原子和分子状态的典型轨迹的一致描述。作为进一步的结果,我们确定了碰撞和辐射弛豫以及光解,自旋翻转碰撞和化学反应的速率。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Life and death of a cold BaRb+ molecule inside an ultracold cloud of Rb atoms
We study the evolution of a single BaRb$^+$ molecule while it continuously collides with ultracold Rb atoms. The initially weakly-bound molecule can undergo a sequence of elastic, inelastic, reactive, and radiative processes. We investigate these processes by developing methods for discriminating between different ion species, electronic states, and kinetic ion energy ranges. By comparing the measurements to model calculations we obtain a consistent description of the typical trajectory of the ion through the manifold of available atomic and molecular states. As a further result, we determine rates for collisional and radiative relaxation as well as photodissociation, spin-flip collisions, and chemical reactions.
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