S. Tashiro, Y. Amano, Kazuo Yoshida, Y. Yamane, G. Uchiyama, H. Abe
{"title":"高活性废液干燥过程中钌的释放特性","authors":"S. Tashiro, Y. Amano, Kazuo Yoshida, Y. Yamane, G. Uchiyama, H. Abe","doi":"10.3327/TAESJ.J14.028","DOIUrl":null,"url":null,"abstract":"The release characteristics of Ru from highly active liquid waste ( HALW ) have been investigated under the condition of accidental evaporation to dryness by boiling of HALW. Using a laboratory-scale apparatus, the simulated HALW ( s - HALW ) was heated with an external heater to dryness to observe the release characteristics of Ru and gaseous nitrogen oxides. As a result, Ru was significantly released between 120 and 300 ℃ of the s - HALW. The cumulative release ratio of Ru was 0.088. It was also found that the partially released amount of Ru against the temperature of the s - HALW had two peaks at about 140 ℃ and about 240 ℃ . Referring to the results of the release rate of gaseous nitrogen oxides and the volume of condensate, which was a collection of the mixed vapors of steam and nitric acid released from the s - HALW, we discussed the causes of Ru release around these peaks.","PeriodicalId":8595,"journal":{"name":"Atomic Energy Society of Japan","volume":"39 1","pages":"227-234"},"PeriodicalIF":0.0000,"publicationDate":"2015-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"4","resultStr":"{\"title\":\"Release Characteristics of Ruthenium from Highly Active Liquid Waste in Drying Step\",\"authors\":\"S. Tashiro, Y. Amano, Kazuo Yoshida, Y. Yamane, G. Uchiyama, H. Abe\",\"doi\":\"10.3327/TAESJ.J14.028\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The release characteristics of Ru from highly active liquid waste ( HALW ) have been investigated under the condition of accidental evaporation to dryness by boiling of HALW. Using a laboratory-scale apparatus, the simulated HALW ( s - HALW ) was heated with an external heater to dryness to observe the release characteristics of Ru and gaseous nitrogen oxides. As a result, Ru was significantly released between 120 and 300 ℃ of the s - HALW. The cumulative release ratio of Ru was 0.088. It was also found that the partially released amount of Ru against the temperature of the s - HALW had two peaks at about 140 ℃ and about 240 ℃ . Referring to the results of the release rate of gaseous nitrogen oxides and the volume of condensate, which was a collection of the mixed vapors of steam and nitric acid released from the s - HALW, we discussed the causes of Ru release around these peaks.\",\"PeriodicalId\":8595,\"journal\":{\"name\":\"Atomic Energy Society of Japan\",\"volume\":\"39 1\",\"pages\":\"227-234\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2015-01-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"4\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Atomic Energy Society of Japan\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.3327/TAESJ.J14.028\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atomic Energy Society of Japan","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.3327/TAESJ.J14.028","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Release Characteristics of Ruthenium from Highly Active Liquid Waste in Drying Step
The release characteristics of Ru from highly active liquid waste ( HALW ) have been investigated under the condition of accidental evaporation to dryness by boiling of HALW. Using a laboratory-scale apparatus, the simulated HALW ( s - HALW ) was heated with an external heater to dryness to observe the release characteristics of Ru and gaseous nitrogen oxides. As a result, Ru was significantly released between 120 and 300 ℃ of the s - HALW. The cumulative release ratio of Ru was 0.088. It was also found that the partially released amount of Ru against the temperature of the s - HALW had two peaks at about 140 ℃ and about 240 ℃ . Referring to the results of the release rate of gaseous nitrogen oxides and the volume of condensate, which was a collection of the mixed vapors of steam and nitric acid released from the s - HALW, we discussed the causes of Ru release around these peaks.