基于光子计数统计的两能级单分子发射光谱

Journal of Atomic and Molecular Sciences Pub Date : 2016-11-01 DOI:10.4208/jams.052316.082216a

Yonggang Peng

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引用次数: 0

摘要

本文介绍了一种获取外场驱动下单分子发射光谱的新方法。引入虚拟探针场来模拟真空场，使受激单分子产生自发发射现象。利用虚探针场引起的发射光子的统计特性，可以得到单分子体系的发射光谱。结果证实了单分子在强外场驱动下的Mollow三重态分裂现象。摘要应提供论文的主要发现的简要总结。pac: 33.50。Dq, 42.50.Ar

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Emission spectrum of two-level single molecule via photon counting statistics

In this paper, we introduce a new way to obtain the emission spectrum of single molecule driven by external field. A virtual probe field is introduced to simulate the vacuum field, which causes the spontaneous emission phenomena of the excited single molecule. The statistical properties of the emission photons caused by the virtual probe field could be used to obtain the emission spectrum of the single molecule system. The results demonstrate the well-known Mollow triplet splitting phenomenon as the single molecule is driven by strong external field.The abstract should provide a brief summary of the main findings of the paper. PACS: 33.50.Dq, 42.50.Ar

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Journal of Atomic and Molecular Sciences PHYSICS, ATOMIC, MOLECULAR & CHEMICAL-

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