Calculation of Critical Experiments involving U(37)O2F2 Solution

Critical experiments were conducted at the Oak Ridge Critical Experiment Facility (ORCEF) to determine the critical concentration for an unreflected 69.2-cm-diameter sphere of UO{sub 2}F{sub 2}, at an enrichment of {approx}37 percent U{sup 235}, by weight. These experiments were a continuation of previous efforts to determine critical dimensions for fissile materials in simple geometry. Some of the earlier experiments in this vessel have been published as part of the OECD handbook. The reports concerning these experiments have only recently become available. Until August 2005, Refs. 2 and 3 were still classified. These documents, along with experimental logbooks and unclassified papers available on the experimental campaign and facility are being used to generate a computer model for this critical experiment.