Wolfgang Loibl, Rudolf Orthofer, Wilfried Winiwarter
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引用次数: 39
摘要
利用排放产生活动的统计信息、技术文献中的排放因子和区域参考数据,计算了奥地利人为非甲烷挥发性有机化合物(NMVOC)的区域排放密度。以1987年为基准年,奥地利人为的NMVOC排放总量估计为467 000公吨。然而,由于可用排放因子的高度不确定性,其范围可能高达316000 - 75.4万t yr−1。人为排放的NMVOC由32%的石蜡、8%的烯烃、20%的芳香族、13%的羰基、6%的光化学“非反应性”和20%的其他化合物组成。基于住区密度、交通密度和相关区域源统计数据,对各源组的总排放量进行了区域分解。在84,000平方公里的面积上总共定义了大约45,000个多边形。虽然奥地利人为NMVOC的理论平均排放密度约为5.6 t km−2 yr−1,但实际排放密度从无人居住地区的0到城市地区的50-100 t km−2 yr−1,以及主要公路沿线的700 t km−2 yr−1不等。因此,全国排放密度平均值无法揭示人口稠密地区的排放密度规模。
Spatially disaggregated emission inventory for anthropogenic NMVOC in Austria
Regional emission densities of anthropogenic non-methane volatile organic compounds (NMVOC) in Austria were calculated using statistical information on emission generation activities, emission factors from technical literature, and regional reference data.
Total anthropogenic NMVOC emissions in Austria were estimated to be 467,000 metric tons for the base year 1987. However, due to the high uncertainties of the available emission factors, the range could be as much as 316,000–754,000 t yr−1. Anthropogenic NMVOC emissions consist of 32% paraffin, 8% olefin, 20% aromatic, 13% carbonyl, 6% photochemically “non-reactive”, and 20% other compounds.
The total emissions from each source group were regionally disaggregated based on settlement densities, traffic densities, and relevant regional source statistics. In total about 45,000 polygons were defined for an area of 84,000 km2. While the theoretical average emission density for anthropogenic NMVOC in Austria would be around 5.6 t km−2 yr−1, the actual emission densities vary from 0 in unpopulated regions to 50–100 t km−2 yr−1 in urban areas and upto 700 t km−2 yr−1 along major highways. National average values for emission densities fail thus to reveal the scale of emission densities in populated areas.