MnFe2O4@g-C3N4纳米复合材料的合成、表征及降解有机污染物的机理

Q1 Earth and Planetary Sciences
Engy Elhaddad , Abdullah T. Al-fawwaz
{"title":"MnFe2O4@g-C3N4纳米复合材料的合成、表征及降解有机污染物的机理","authors":"Engy Elhaddad ,&nbsp;Abdullah T. Al-fawwaz","doi":"10.1016/j.ejpe.2023.05.002","DOIUrl":null,"url":null,"abstract":"<div><p>Photocatalysis has recently been shown to be a good way to get rid of pollutants and produce hydrogen. MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> was synthesized by solid state synthesis technique. In addition to producing hydrogen, MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> demonstrated outstanding photocatalytic performance for the decay of pesticides under visible illumination. The morphology and structure of MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> were approved using Scanning Electron Microscopes (SEM), X-ray diffraction (XRD). Morover, Fourier transform infrared spectroscopy (FT-IR), UV–vis DRS, and surface area (BET). Based on the degradation of the carbaryl contaminant, the photocatalytic action of MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> was evaluated (94%). We for the first time could generate hydrogen by MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> and develop its photocatalytic activities by expanding the surface area and narrowing the band gap value (1.7 eV) and a great surface area of 53.46 m<sup>2</sup>/g, as displayed by the outcomes.</p></div>","PeriodicalId":11625,"journal":{"name":"Egyptian Journal of Petroleum","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2023-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Synthesis, Characterization and Mechanism of MnFe2O4@g-C3N4 Nanocomposite as an effective Photocatalyst for the Generation of Hydrogen and organic contamination degradation\",\"authors\":\"Engy Elhaddad ,&nbsp;Abdullah T. Al-fawwaz\",\"doi\":\"10.1016/j.ejpe.2023.05.002\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Photocatalysis has recently been shown to be a good way to get rid of pollutants and produce hydrogen. MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> was synthesized by solid state synthesis technique. In addition to producing hydrogen, MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> demonstrated outstanding photocatalytic performance for the decay of pesticides under visible illumination. The morphology and structure of MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> were approved using Scanning Electron Microscopes (SEM), X-ray diffraction (XRD). Morover, Fourier transform infrared spectroscopy (FT-IR), UV–vis DRS, and surface area (BET). Based on the degradation of the carbaryl contaminant, the photocatalytic action of MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> was evaluated (94%). We for the first time could generate hydrogen by MnFe<sub>2</sub>O<sub>4</sub>@g-C<sub>3</sub>N<sub>4</sub> and develop its photocatalytic activities by expanding the surface area and narrowing the band gap value (1.7 eV) and a great surface area of 53.46 m<sup>2</sup>/g, as displayed by the outcomes.</p></div>\",\"PeriodicalId\":11625,\"journal\":{\"name\":\"Egyptian Journal of Petroleum\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2023-06-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Egyptian Journal of Petroleum\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1110062123000235\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"Earth and Planetary Sciences\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Egyptian Journal of Petroleum","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1110062123000235","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Earth and Planetary Sciences","Score":null,"Total":0}
引用次数: 0

摘要

光催化最近被证明是一种去除污染物和产生氢的好方法。MnFe2O4@g-C3N4是通过固态合成技术合成的。除了产生氢气外,MnFe2O4@g-C3N4在可见光照明下对农药的衰变表现出出色的光催化性能。利用扫描电子显微镜(SEM)、x射线衍射仪(XRD)对MnFe2O4@g-C3N4的形貌和结构进行了表征。此外,傅里叶变换红外光谱(FT-IR), UV-vis DRS和表面积(BET)。基于对西维因污染物的降解,评价了MnFe2O4@g-C3N4的光催化作用(94%)。结果表明,我们首次可以通过MnFe2O4@g-C3N4生成氢气,并通过扩大表面积和缩小带隙值(1.7 eV)和53.46 m2/g的大表面积来开发其光催化活性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Synthesis, Characterization and Mechanism of MnFe2O4@g-C3N4 Nanocomposite as an effective Photocatalyst for the Generation of Hydrogen and organic contamination degradation

Photocatalysis has recently been shown to be a good way to get rid of pollutants and produce hydrogen. MnFe2O4@g-C3N4 was synthesized by solid state synthesis technique. In addition to producing hydrogen, MnFe2O4@g-C3N4 demonstrated outstanding photocatalytic performance for the decay of pesticides under visible illumination. The morphology and structure of MnFe2O4@g-C3N4 were approved using Scanning Electron Microscopes (SEM), X-ray diffraction (XRD). Morover, Fourier transform infrared spectroscopy (FT-IR), UV–vis DRS, and surface area (BET). Based on the degradation of the carbaryl contaminant, the photocatalytic action of MnFe2O4@g-C3N4 was evaluated (94%). We for the first time could generate hydrogen by MnFe2O4@g-C3N4 and develop its photocatalytic activities by expanding the surface area and narrowing the band gap value (1.7 eV) and a great surface area of 53.46 m2/g, as displayed by the outcomes.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Egyptian Journal of Petroleum
Egyptian Journal of Petroleum Earth and Planetary Sciences-Geochemistry and Petrology
CiteScore
7.70
自引率
0.00%
发文量
29
审稿时长
84 days
期刊介绍: Egyptian Journal of Petroleum is addressed to the fields of crude oil, natural gas, energy and related subjects. Its objective is to serve as a forum for research and development covering the following areas: • Sedimentation and petroleum exploration. • Production. • Analysis and testing. • Chemistry and technology of petroleum and natural gas. • Refining and processing. • Catalysis. • Applications and petrochemicals. It also publishes original research papers and reviews in areas relating to synthetic fuels and lubricants - pollution - corrosion - alternate sources of energy - gasification, liquefaction and geology of coal - tar sands and oil shale - biomass as a source of renewable energy. To meet with these requirements the Egyptian Journal of Petroleum welcomes manuscripts and review papers reporting on the state-of-the-art in the aforementioned topics. The Egyptian Journal of Petroleum is also willing to publish the proceedings of petroleum and energy related conferences in a single volume form.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信