走向实用的圆偏振发光:基于碳点的圆偏振激光器

IF 13.5 2区 化学 Q1 CHEMISTRY, PHYSICAL
物理化学学报 Pub Date : 2026-04-01 Epub Date: 2025-09-24 DOI:10.1016/j.actphy.2025.100191
Ting Li , Xiao Zeng , Yuzhuo Yang , Xinyi Wen, Shurong Ding, Linlin Shi, Yongqiang Zhang, Siyu Lu
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引用次数: 0

摘要

圆偏光在量子计算、三维显示、生物成像等领域具有重要的应用价值。然而,其实际应用面临着不对称因子(g)低、量子产率不足、方向性差、发射光谱宽等挑战。针对这些问题,圆偏振光技术可以通过受激发射放大和谐振腔模式选择,显著提高CPL性能,实现高g(接近2的理论极限)、高亮度、窄线宽、强方向性的圆偏振光输出。目前,有机微晶体、钙钛矿等材料虽然可以实现高g的圆偏振激光,但仍存在制备复杂、生物相容性差等问题。而碳点(cd)由于其制备简单、成本低、毒性小、易修饰、生物相容性好等优点,成为一种极具发展前景的新型圆极化增益介质。本文系统地综述了圆偏振激光器的材料体系、器件类型和应用进展,重点介绍了圆偏振激光器作为增益介质的优势及其在三维显示、光通信、信息加密、生物传感等领域的应用潜力。展望了基于cd的圆偏光激光器未来的发展方向和面临的挑战,为推动高性能圆偏光器件的实际应用进程提供参考。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Towards practical circularly polarized luminescence: Carbon dots-based circularly polarized lasers

Towards practical circularly polarized luminescence: Carbon dots-based circularly polarized lasers
Circularly polarized luminescence (CPL) has significant application value in fields such as quantum computing, three-dimensional (3D) display, and bioimaging. However, its practical application faces challenges including low dissymmetry factor (g), insufficient quantum yield, poor directionality, and broad emission spectrum. To address these issues, circularly polarized laser technology can significantly enhance CPL performance through stimulated emission amplification and resonant cavity mode selection, achieving circularly polarized light output with high g (close to the theoretical limit of 2), high brightness, narrow linewidth, and strong directionality. Currently, although materials like organic microcrystals and perovskites can realize circularly polarized laser with high g, they still have problems such as complex preparation and poor biocompatibility. In contrast, carbon dots (CDs) have emerged as a highly promising new type of circularly polarized gain medium due to their advantages of simple preparation, low cost, low toxicity, easy modification, and good biocompatibility. This paper systematically reviews the material systems, device types, and application progress of circularly polarized laser, focusing on the advantages of CDs as gain media and their potential in fields such as 3D display, optical communication, information encryption, and biosensing. It also prospects the future development directions and challenges of CDs-based circularly polarized lasers, providing a reference for promoting the practical application process of high-performance circularly polarized laser devices.
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来源期刊
物理化学学报
物理化学学报 化学-物理化学
CiteScore
16.60
自引率
5.50%
发文量
9754
审稿时长
1.2 months
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