低温下亚纳秒激光脉冲刺激下金刚石发光特性的变化

IF 0.6 4区 物理与天体物理 Q4 PHYSICS, MULTIDISCIPLINARY
S. I. Chentsov, I. I. Usmanov, V. S. Krivobok
{"title":"低温下亚纳秒激光脉冲刺激下金刚石发光特性的变化","authors":"S. I. Chentsov,&nbsp;I. I. Usmanov,&nbsp;V. S. Krivobok","doi":"10.3103/S1068335625600020","DOIUrl":null,"url":null,"abstract":"<p>The effect of 532-nm pulsed laser radiation on properties of a single-crystal diamond film containing optically active SiV<sup>‒</sup> centers is studied using in-situ measurements of the photoluminescence spectra at a temperature of 77 K. It is shown that at a pulse duration of 500 ns, the threshold energy density at which the rearrangement of SiV<sup>‒</sup> centers is recorded is ~0.112 J/cm<sup>2</sup>. The rearrangement leads to a decrease in the intensity of the zero-phonon emission line of SiV<sup>‒</sup> centers relative to the intensity of the Raman scattering signal on optical phonons of the diamond matrix. With an increase in the energy density of incident pulses to 0.540 J/cm<sup>2</sup>, the luminescence quenching effect reaches saturation, and traces of ablation and/or graphitization are observed on the film surface. The found effects are explained by local heating of the diamond film due to the processes of three-photon absorption of light, in which the absorption coefficient sharply depends on the energy of incident pulses.</p>","PeriodicalId":503,"journal":{"name":"Bulletin of the Lebedev Physics Institute","volume":"52 3","pages":"107 - 113"},"PeriodicalIF":0.6000,"publicationDate":"2025-04-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Change in Luminescent Properties of Diamond Stimulated by Subnanosecond Laser Pulses at Low Temperatures\",\"authors\":\"S. I. Chentsov,&nbsp;I. I. Usmanov,&nbsp;V. S. Krivobok\",\"doi\":\"10.3103/S1068335625600020\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>The effect of 532-nm pulsed laser radiation on properties of a single-crystal diamond film containing optically active SiV<sup>‒</sup> centers is studied using in-situ measurements of the photoluminescence spectra at a temperature of 77 K. It is shown that at a pulse duration of 500 ns, the threshold energy density at which the rearrangement of SiV<sup>‒</sup> centers is recorded is ~0.112 J/cm<sup>2</sup>. The rearrangement leads to a decrease in the intensity of the zero-phonon emission line of SiV<sup>‒</sup> centers relative to the intensity of the Raman scattering signal on optical phonons of the diamond matrix. With an increase in the energy density of incident pulses to 0.540 J/cm<sup>2</sup>, the luminescence quenching effect reaches saturation, and traces of ablation and/or graphitization are observed on the film surface. The found effects are explained by local heating of the diamond film due to the processes of three-photon absorption of light, in which the absorption coefficient sharply depends on the energy of incident pulses.</p>\",\"PeriodicalId\":503,\"journal\":{\"name\":\"Bulletin of the Lebedev Physics Institute\",\"volume\":\"52 3\",\"pages\":\"107 - 113\"},\"PeriodicalIF\":0.6000,\"publicationDate\":\"2025-04-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Bulletin of the Lebedev Physics Institute\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://link.springer.com/article/10.3103/S1068335625600020\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"PHYSICS, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Bulletin of the Lebedev Physics Institute","FirstCategoryId":"101","ListUrlMain":"https://link.springer.com/article/10.3103/S1068335625600020","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

研究了532 nm脉冲激光辐射对含有光学活性SiV中心的单晶金刚石薄膜性能的影响,并在77 K的温度下进行了原位光致发光光谱测量。结果表明,在脉冲持续时间为500 ns时,记录SiV中心重排的阈值能量密度为~0.112 J/cm2。这种重排导致SiV -中心的零声子发射线的强度相对于金刚石基体光学声子上的拉曼散射信号的强度降低。当入射脉冲的能量密度增加到0.540 J/cm2时,薄膜的发光猝灭达到饱和,薄膜表面出现烧蚀和石墨化现象。所发现的效应可以用金刚石薄膜的局部加热来解释,这是由于光的三光子吸收过程,其中吸收系数与入射脉冲的能量密切相关。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Change in Luminescent Properties of Diamond Stimulated by Subnanosecond Laser Pulses at Low Temperatures

The effect of 532-nm pulsed laser radiation on properties of a single-crystal diamond film containing optically active SiV centers is studied using in-situ measurements of the photoluminescence spectra at a temperature of 77 K. It is shown that at a pulse duration of 500 ns, the threshold energy density at which the rearrangement of SiV centers is recorded is ~0.112 J/cm2. The rearrangement leads to a decrease in the intensity of the zero-phonon emission line of SiV centers relative to the intensity of the Raman scattering signal on optical phonons of the diamond matrix. With an increase in the energy density of incident pulses to 0.540 J/cm2, the luminescence quenching effect reaches saturation, and traces of ablation and/or graphitization are observed on the film surface. The found effects are explained by local heating of the diamond film due to the processes of three-photon absorption of light, in which the absorption coefficient sharply depends on the energy of incident pulses.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Bulletin of the Lebedev Physics Institute
Bulletin of the Lebedev Physics Institute PHYSICS, MULTIDISCIPLINARY-
CiteScore
0.70
自引率
25.00%
发文量
41
审稿时长
6-12 weeks
期刊介绍: Bulletin of the Lebedev Physics Institute is an international peer reviewed journal that publishes results of new original experimental and theoretical studies on all topics of physics: theoretical physics; atomic and molecular physics; nuclear physics; optics; lasers; condensed matter; physics of solids; biophysics, and others.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信