废物转化为资源:用等离子体处理的碳纤维增强氢的释放

Wenyan Zhang , Weidong Tao , Yihan Wang , Chaoqun Jiang , Hangmin Guan , Yingfei Hu , Wenjie Tian , Linyun Hao
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引用次数: 0

摘要

全球对化石燃料的依赖日益增加,导致了重大的能源危机和环境问题,凸显了对氢等可再生能源的迫切需求。本研究提出了等离子体处理的碳纤维负载Pt (P-CF@Pt),以改善光催化析氢。等离子体处理产生的表面官能团增强了碳纤维(CFs)的亲水性,促进了液体反应系统中更好的分散,并促进了铂的负载。经过处理的CF表面和Pt位点之间的这种相互作用显著地促进了电荷分离和催化性能,从而提高了光电压,降低了质子还原的起始电位,增强了电子传递。与未经处理的CF相比,P-CF@Pt复合材料表现出更好的光催化效率,氢产量增加23%。这些发现强调了利用等离子体处理的CFs开发具有成本效益和可扩展的光催化制氢系统的前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Transforming waste into resource: Enhanced hydrogen evolution with plasma-treated carbon fiber

Transforming waste into resource: Enhanced hydrogen evolution with plasma-treated carbon fiber
The increasing global dependence on fossil fuels has led to significant energy crises and environmental issues, highlighting the urgent need for renewable energy sources such as hydrogen. This study presents the development of plasma-treated carbon fiber loaded with Pt (P-CF@Pt) to improve photocatalytic hydrogen evolution. The plasma treatment creates surface functional groups that enhance the hydrophilicity of the carbon fibers (CFs), promoting better dispersion in liquid reaction systems and facilitating Pt loading. This interaction between the treated CF surface and the Pt sites significantly boosts charge separation and catalytic performance, resulting in improved photovoltage, lower onset potential for proton reduction, and enhanced electron transport. The P-CF@Pt composite demonstrates better photocatalytic efficiency compared to untreated CF, achieving a 23% increase in hydrogen production. These findings underscore the promise of utilizing plasma-treated CFs in the development of cost-effective and scalable photocatalytic systems for hydrogen generation.
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