全印刷场效应晶体管湿度传感器,壳聚糖/聚乙烯醇/纳米碳粉增强湿度敏感性。

IF 5.6 1区 化学 Q1 CHEMISTRY, ANALYTICAL
Talanta Pub Date : 2025-05-15 Epub Date: 2025-02-03 DOI:10.1016/j.talanta.2025.127679
Ruifang Liu, Zhenting Wu, Qiang Li, Sara Shamim, Long Ba
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引用次数: 0

摘要

随着柔性电子技术的进步,可穿戴设备对低成本、高性能柔性湿度传感器的需求显著增加。然而,商用湿度传感器需要复杂的制备方法,而且价格昂贵。因此,我们报道了聚乙烯醇/壳聚糖/纳米碳粉(PVA/CS/NCP)湿度敏感复合材料,并通过扫描电子显微镜(SEM)、傅里叶变换红外光谱(FTIR)和接触角测量对其进行了表征。采用丝网印刷技术制作了一种电阻式湿度传感器,该传感器在33%RH-98%RH湿度下具有良好的响应,在98%RH湿度下,传感器的响应达到1.74。通过将离子凝胶晶体管与CS/PVA/NCP湿敏电阻集成,制备了全印刷场效应晶体管(FET)湿度传感器。对比表明,FET湿度传感器的响应显著提高,在98% RH下达到6.27。此外,两种类型的传感器都具有较小的滞后和良好的可重复性。最后,我们在非接触和可变呼吸条件下测试了构建的湿度传感器,为未来的可穿戴应用奠定了基础。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Fully printed field-effect transistor humidity sensor with chitosan/polyvinyl alcohol/nano carbon powder for enhanced moisture sensitivity.

With the advancement of flexible electronics, the demand for low-cost, high-performance flexible humidity sensors for wearable devices has increased significantly. However, commercial humidity sensors require complex preparation methods and are expensive. Therefore, we report polyvinyl alcohol/chitosan/nano carbon powder (PVA/CS/NCP) humidity-sensitive composite materials, which were characterized by scanning electron microscopy (SEM), Fourier transform infrared spectroscopy (FTIR), and contact angle measurements. A resistive humidity sensor was fabricated using screen printing, and the device showed a good response at 33%RH-98%RH humidity, and at 98 % RH, the sensor achieved a response of 1.74. A fully printed field-effect transistor (FET) humidity sensor was prepared by integrating an ion gel transistor with a CS/PVA/NCP humidity-sensitive resistor to improve the response. The comparison reveals a significant improvement in the FET humidity sensor's response, reaching 6.27 at 98 % RH. In addition, both types of sensors exhibit less hysteresis and good repeatability. Lastly, we tested the constructed humidity sensors under non-contact and variable breathing conditions, laying the groundwork for future wearable applications.

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来源期刊
Talanta
Talanta 化学-分析化学
CiteScore
12.30
自引率
4.90%
发文量
861
审稿时长
29 days
期刊介绍: Talanta provides a forum for the publication of original research papers, short communications, and critical reviews in all branches of pure and applied analytical chemistry. Papers are evaluated based on established guidelines, including the fundamental nature of the study, scientific novelty, substantial improvement or advantage over existing technology or methods, and demonstrated analytical applicability. Original research papers on fundamental studies, and on novel sensor and instrumentation developments, are encouraged. Novel or improved applications in areas such as clinical and biological chemistry, environmental analysis, geochemistry, materials science and engineering, and analytical platforms for omics development are welcome. Analytical performance of methods should be determined, including interference and matrix effects, and methods should be validated by comparison with a standard method, or analysis of a certified reference material. Simple spiking recoveries may not be sufficient. The developed method should especially comprise information on selectivity, sensitivity, detection limits, accuracy, and reliability. However, applying official validation or robustness studies to a routine method or technique does not necessarily constitute novelty. Proper statistical treatment of the data should be provided. Relevant literature should be cited, including related publications by the authors, and authors should discuss how their proposed methodology compares with previously reported methods.
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