太湖表层沉积物中有机紫外线吸收物的赋存、空间分布及生态风险

IF 6.9 2区环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES

Emerging Contaminants Pub Date : 2025-01-02 DOI:10.1016/j.emcon.2024.100466

Wen Gu , Shuai Sun , Yinying Cai , Ziyan Du , Xiaohan Shan , Mengyuan Liang , Min Guo , Linjun Zhou , Yong Zhang

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引用次数: 0

摘要

研究了太湖表层沉积物中8种有机紫外线吸收剂的赋存状态和空间分布特征。2016年uva的检测频率和浓度均显著高于2015年，其中以甲氧基肉桂酸乙己酯和高盐酸酯（HMS）为主。沉积物样品中UVA总浓度范围为0.15 ~ 85.3 ng/g。空间分布结果表明，uva主要集中在太湖西北部。总有机碳含量可能影响uva在沉积物中的命运。来源分析和相关分析表明，2015年2-乙基己基甲氧基肉桂酸酯、水杨酸乙基己基和HMS占比高且相关性显著；以及二苯甲酮-3、HMS和水杨酸苄酯。这些结果表明，每年的相关化合物具有相同的来源。生态风险评价结果表明，太湖沉积物中uva对底栖生物具有中等风险。2016年uva风险系数略高于2015年。uva的季节性污染特征及其综合环境风险值得进一步关注。

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Occurrences, spatial distributions, and ecological risks of organic ultraviolet absorbents in surface sediments from Taihu Lake, China

The occurrences and spatial distributions of eight organic ultraviolet absorbents (UVAs) were investigated in surface sediments from Taihu Lake, China. The detection frequencies and concentrations of UVAs in 2016 were significantly higher than those in 2015.2-Ethylhexyl methoxycinnamate and homosalate (HMS) were the predominant UVAs in the sediment samples. The total UVA concentration range in sediment samples was 0.15–85.3 ng/g. The spatial distribution results showed that UVAs were concentrated in the northwest of Taihu Lake. The total organic carbon content may affect the fate of UVAs in sediments. Source analysis and correlation analysis showed that the following compounds had high proportions and significant correlations: 2-ethylhexyl methoxycinnamate, ethylhexyl salicylate, and HMS in 2015; and benzophenone-3, HMS, and benzyl salicylate in 2016. These results indicated the correlated compounds within each year had the same source. Ecological risk assessment results showed that UVAs in sediment from Taihu Lake may present a moderate risk to benthic organisms. The risk quotient of UVAs in 2016 was slightly higher than that in 2015. The seasonal pollution characteristics of UVAs and their comprehensive environmental risks should receive further attention.

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来源期刊

Emerging Contaminants Medicine-Public Health, Environmental and Occupational Health

CiteScore

10.00

自引率

6.70%

发文量

审稿时长

44 days

期刊介绍： Emerging Contaminants is an outlet for world-leading research addressing problems associated with environmental contamination caused by emerging contaminants and their solutions. Emerging contaminants are defined as chemicals that are not currently (or have been only recently) regulated and about which there exist concerns regarding their impact on human or ecological health. Examples of emerging contaminants include disinfection by-products, pharmaceutical and personal care products, persistent organic chemicals, and mercury etc. as well as their degradation products. We encourage papers addressing science that facilitates greater understanding of the nature, extent, and impacts of the presence of emerging contaminants in the environment; technology that exploits original principles to reduce and control their environmental presence; as well as the development, implementation and efficacy of national and international policies to protect human health and the environment from emerging contaminants.