Chao Li
(, ), Hong Yan
(, ), Hanlu Yang
(, ), Wenqian Zhou
(, ), Chengyu Xie
(, ), Baocai Pan
(, ), Qichun Zhang
(, )
{"title":"金属-有机骨架作为高效二氧化碳还原电催化剂的研究进展与展望","authors":"Chao Li \n (, ), Hong Yan \n (, ), Hanlu Yang \n (, ), Wenqian Zhou \n (, ), Chengyu Xie \n (, ), Baocai Pan \n (, ), Qichun Zhang \n (, )","doi":"10.1007/s40843-024-3165-6","DOIUrl":null,"url":null,"abstract":"<div><p>The conversion of carbon dioxide (CO<sub>2</sub>) to the reduced chemical compounds offers substantial environmental benefits through minimizing the emission of greenhouse gas and fostering sustainable practices. Recently, the unique properties of metal-organic frameworks (MOFs) make them attractive candidates for electrocatalytic CO<sub>2</sub> reduction reaction (CO<sub>2</sub>RR), providing many opportunities to develop efficient, selective, and environmentally sustainable processes for mitigating CO<sub>2</sub> emissions and utilizing CO<sub>2</sub> as a valuable raw material for the synthesis of fuels and chemicals. Here, the recent advances in MOFs as efficient catalysts for electrocatalytic CO<sub>2</sub>RR are summarized. The detailed characteristics, electrocatalytic mechanisms, and practical approaches for improving the electrocatalytic efficiency, selectivity, and durability of MOFs under realistic reaction conditions are also clarified. Furthermore, the outlooks on the prospects of MOF-based electrocatalysts in CO<sub>2</sub>RR are provided.</p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>","PeriodicalId":773,"journal":{"name":"Science China Materials","volume":"68 1","pages":"21 - 38"},"PeriodicalIF":6.8000,"publicationDate":"2024-11-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40843-024-3165-6.pdf","citationCount":"0","resultStr":"{\"title\":\"Recent advances and future perspectives of metal-organic frameworks as efficient electrocatalysts for CO2 reduction\",\"authors\":\"Chao Li \\n (, ), Hong Yan \\n (, ), Hanlu Yang \\n (, ), Wenqian Zhou \\n (, ), Chengyu Xie \\n (, ), Baocai Pan \\n (, ), Qichun Zhang \\n (, )\",\"doi\":\"10.1007/s40843-024-3165-6\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The conversion of carbon dioxide (CO<sub>2</sub>) to the reduced chemical compounds offers substantial environmental benefits through minimizing the emission of greenhouse gas and fostering sustainable practices. Recently, the unique properties of metal-organic frameworks (MOFs) make them attractive candidates for electrocatalytic CO<sub>2</sub> reduction reaction (CO<sub>2</sub>RR), providing many opportunities to develop efficient, selective, and environmentally sustainable processes for mitigating CO<sub>2</sub> emissions and utilizing CO<sub>2</sub> as a valuable raw material for the synthesis of fuels and chemicals. Here, the recent advances in MOFs as efficient catalysts for electrocatalytic CO<sub>2</sub>RR are summarized. The detailed characteristics, electrocatalytic mechanisms, and practical approaches for improving the electrocatalytic efficiency, selectivity, and durability of MOFs under realistic reaction conditions are also clarified. Furthermore, the outlooks on the prospects of MOF-based electrocatalysts in CO<sub>2</sub>RR are provided.</p><div><figure><div><div><picture><source><img></source></picture></div></div></figure></div></div>\",\"PeriodicalId\":773,\"journal\":{\"name\":\"Science China Materials\",\"volume\":\"68 1\",\"pages\":\"21 - 38\"},\"PeriodicalIF\":6.8000,\"publicationDate\":\"2024-11-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://link.springer.com/content/pdf/10.1007/s40843-024-3165-6.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Science China Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s40843-024-3165-6\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Science China Materials","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s40843-024-3165-6","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Recent advances and future perspectives of metal-organic frameworks as efficient electrocatalysts for CO2 reduction
The conversion of carbon dioxide (CO2) to the reduced chemical compounds offers substantial environmental benefits through minimizing the emission of greenhouse gas and fostering sustainable practices. Recently, the unique properties of metal-organic frameworks (MOFs) make them attractive candidates for electrocatalytic CO2 reduction reaction (CO2RR), providing many opportunities to develop efficient, selective, and environmentally sustainable processes for mitigating CO2 emissions and utilizing CO2 as a valuable raw material for the synthesis of fuels and chemicals. Here, the recent advances in MOFs as efficient catalysts for electrocatalytic CO2RR are summarized. The detailed characteristics, electrocatalytic mechanisms, and practical approaches for improving the electrocatalytic efficiency, selectivity, and durability of MOFs under realistic reaction conditions are also clarified. Furthermore, the outlooks on the prospects of MOF-based electrocatalysts in CO2RR are provided.
期刊介绍：
Science China Materials (SCM) is a globally peer-reviewed journal that covers all facets of materials science. It is supervised by the Chinese Academy of Sciences and co-sponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China. The journal is jointly published monthly in both printed and electronic forms by Science China Press and Springer. The aim of SCM is to encourage communication of high-quality, innovative research results at the cutting-edge interface of materials science with chemistry, physics, biology, and engineering. It focuses on breakthroughs from around the world and aims to become a world-leading academic journal for materials science.
求助内容：
应助结果提醒方式：
京公网安备 11010802042870号
