{"title":"用于 DAC 的二氧化碳吸附教学模型：波浪解决方案和最佳流程。","authors":"Emily Kay-Leighton, Henning Struchtrup","doi":"10.3390/e26110972","DOIUrl":null,"url":null,"abstract":"<p><p>We present and investigate a simple yet instructive model for the adsorption of CO<sub>2</sub> from air in porous media as used in direct air capture (DAC) processes. Mathematical analysis and non-dimensionalization reveal that the sorbent is characterized by the sorption timescale and capacity, while the adsorption process is effectively wavelike. The systematic evaluation shows that the overall adsorption rate and the recommended charging duration depend only on the wave parameter that is found as the ratio of capacity and dimensionless air flow velocity. Specifically, smaller wave parameters yield a larger overall charging rate, while larger wave parameters reduce the work required to move air through the sorbent. Thus, optimal process conditions must compromise between a large overall adsorption rate and low work requirements.</p>","PeriodicalId":11694,"journal":{"name":"Entropy","volume":"26 11","pages":""},"PeriodicalIF":2.1000,"publicationDate":"2024-11-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11593035/pdf/","citationCount":"0","resultStr":"{\"title\":\"An Instructive CO<sub>2</sub> Adsorption Model for DAC: Wave Solutions and Optimal Processes.\",\"authors\":\"Emily Kay-Leighton, Henning Struchtrup\",\"doi\":\"10.3390/e26110972\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>We present and investigate a simple yet instructive model for the adsorption of CO<sub>2</sub> from air in porous media as used in direct air capture (DAC) processes. Mathematical analysis and non-dimensionalization reveal that the sorbent is characterized by the sorption timescale and capacity, while the adsorption process is effectively wavelike. The systematic evaluation shows that the overall adsorption rate and the recommended charging duration depend only on the wave parameter that is found as the ratio of capacity and dimensionless air flow velocity. Specifically, smaller wave parameters yield a larger overall charging rate, while larger wave parameters reduce the work required to move air through the sorbent. Thus, optimal process conditions must compromise between a large overall adsorption rate and low work requirements.</p>\",\"PeriodicalId\":11694,\"journal\":{\"name\":\"Entropy\",\"volume\":\"26 11\",\"pages\":\"\"},\"PeriodicalIF\":2.1000,\"publicationDate\":\"2024-11-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11593035/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Entropy\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.3390/e26110972\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"PHYSICS, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Entropy","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.3390/e26110972","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
An Instructive CO2 Adsorption Model for DAC: Wave Solutions and Optimal Processes.
We present and investigate a simple yet instructive model for the adsorption of CO2 from air in porous media as used in direct air capture (DAC) processes. Mathematical analysis and non-dimensionalization reveal that the sorbent is characterized by the sorption timescale and capacity, while the adsorption process is effectively wavelike. The systematic evaluation shows that the overall adsorption rate and the recommended charging duration depend only on the wave parameter that is found as the ratio of capacity and dimensionless air flow velocity. Specifically, smaller wave parameters yield a larger overall charging rate, while larger wave parameters reduce the work required to move air through the sorbent. Thus, optimal process conditions must compromise between a large overall adsorption rate and low work requirements.
期刊介绍：
Entropy (ISSN 1099-4300), an international and interdisciplinary journal of entropy and information studies, publishes reviews, regular research papers and short notes. Our aim is to encourage scientists to publish as much as possible their theoretical and experimental details. There is no restriction on the length of the papers. If there are computation and the experiment, the details must be provided so that the results can be reproduced.
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