Xiang Song, Haonan Peng, Jianmin Zhang, Xiaolong He
{"title":"液滴撞击非均匀化学图案燃料电池表面的能量演化","authors":"Xiang Song, Haonan Peng, Jianmin Zhang, Xiaolong He","doi":"10.1016/j.ces.2024.120887","DOIUrl":null,"url":null,"abstract":"<div><div>A three-dimensional nonorthogonal lattice Boltzmann model is employed to simulate a single droplet impacting a nonuniform wettable surface at the bottom of a proton exchange membrane fuel cell. The effects of nonuniform surface wettability differences in the flow channel, the impact Weber number, and the central stripe width on the energy evolution during the spreading stage are investigated. Qualitative and quantitative comparisons between the numerical simulations and experimental results indicate that the main energy loss during the initial spreading stage is attributable to momentum redistribution, while viscous dissipation is caused by shear stress and vorticity in the rim. A larger wettability difference leads to a higher net unbalanced Young’s force, resulting in stronger shear and viscous dissipation near the wettability contrast line. For smaller Weber numbers, in the early impact stage, the main loss of kinetic energy is caused by the redistribution of momentum; in the later spreading stage, the increase in surface energy is the main sink of kinetic energy. The unbalanced Young’s force hinders the spreading of the droplet at larger stripe widths, leading to a larger vortex intensity within the rim.</div></div>","PeriodicalId":271,"journal":{"name":"Chemical Engineering Science","volume":"302 ","pages":"Article 120887"},"PeriodicalIF":4.1000,"publicationDate":"2024-11-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Energy evolution of a droplet impacting a nonuniform chemically patterned fuel cell surface\",\"authors\":\"Xiang Song, Haonan Peng, Jianmin Zhang, Xiaolong He\",\"doi\":\"10.1016/j.ces.2024.120887\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>A three-dimensional nonorthogonal lattice Boltzmann model is employed to simulate a single droplet impacting a nonuniform wettable surface at the bottom of a proton exchange membrane fuel cell. The effects of nonuniform surface wettability differences in the flow channel, the impact Weber number, and the central stripe width on the energy evolution during the spreading stage are investigated. Qualitative and quantitative comparisons between the numerical simulations and experimental results indicate that the main energy loss during the initial spreading stage is attributable to momentum redistribution, while viscous dissipation is caused by shear stress and vorticity in the rim. A larger wettability difference leads to a higher net unbalanced Young’s force, resulting in stronger shear and viscous dissipation near the wettability contrast line. For smaller Weber numbers, in the early impact stage, the main loss of kinetic energy is caused by the redistribution of momentum; in the later spreading stage, the increase in surface energy is the main sink of kinetic energy. The unbalanced Young’s force hinders the spreading of the droplet at larger stripe widths, leading to a larger vortex intensity within the rim.</div></div>\",\"PeriodicalId\":271,\"journal\":{\"name\":\"Chemical Engineering Science\",\"volume\":\"302 \",\"pages\":\"Article 120887\"},\"PeriodicalIF\":4.1000,\"publicationDate\":\"2024-11-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Engineering Science\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0009250924011874\",\"RegionNum\":2,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Science","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0009250924011874","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
Energy evolution of a droplet impacting a nonuniform chemically patterned fuel cell surface
A three-dimensional nonorthogonal lattice Boltzmann model is employed to simulate a single droplet impacting a nonuniform wettable surface at the bottom of a proton exchange membrane fuel cell. The effects of nonuniform surface wettability differences in the flow channel, the impact Weber number, and the central stripe width on the energy evolution during the spreading stage are investigated. Qualitative and quantitative comparisons between the numerical simulations and experimental results indicate that the main energy loss during the initial spreading stage is attributable to momentum redistribution, while viscous dissipation is caused by shear stress and vorticity in the rim. A larger wettability difference leads to a higher net unbalanced Young’s force, resulting in stronger shear and viscous dissipation near the wettability contrast line. For smaller Weber numbers, in the early impact stage, the main loss of kinetic energy is caused by the redistribution of momentum; in the later spreading stage, the increase in surface energy is the main sink of kinetic energy. The unbalanced Young’s force hinders the spreading of the droplet at larger stripe widths, leading to a larger vortex intensity within the rim.
期刊介绍:
Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline.
Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.