人工孢子作为多功能生物催化剂执行生物合成级联(功能材料学进展 45/2024)

IF 18.5 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Maialen Iturralde, Magdalena Ripoll, Desiré di Silvio, Marta Gallego, Daniel A. Grajales-Hernández, Xabier López, Lorena Betancor, Fernando López-Gallego
{"title":"人工孢子作为多功能生物催化剂执行生物合成级联(功能材料学进展 45/2024)","authors":"Maialen Iturralde,&nbsp;Magdalena Ripoll,&nbsp;Desiré di Silvio,&nbsp;Marta Gallego,&nbsp;Daniel A. Grajales-Hernández,&nbsp;Xabier López,&nbsp;Lorena Betancor,&nbsp;Fernando López-Gallego","doi":"10.1002/adfm.202470261","DOIUrl":null,"url":null,"abstract":"<p><b>Enzyme Immobilization</b></p><p>In article number 2406097, Fernando López-Gallego and co-workers develop a universal method for encapsulating single gram-negative microbes with polymeric coatings to fabricate synthetic spores that selectively bind His-tagged enzymes. These synthetic spores serve as biocatalytic materials for the one-pot oxidative amination of diols into amino alcohols, facilitated by the cooperative catalysis between intracellular and extracellular enzymes that maintain their performance in consecutive batch cycles.\n\n <figure>\n <div><picture>\n <source></source></picture><p></p>\n </div>\n </figure></p>","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":null,"pages":null},"PeriodicalIF":18.5000,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adfm.202470261","citationCount":"0","resultStr":"{\"title\":\"Artificial Spores as Multi-Functional Biocatalysts to Perform Biosynthetic Cascades (Adv. Funct. Mater. 45/2024)\",\"authors\":\"Maialen Iturralde,&nbsp;Magdalena Ripoll,&nbsp;Desiré di Silvio,&nbsp;Marta Gallego,&nbsp;Daniel A. Grajales-Hernández,&nbsp;Xabier López,&nbsp;Lorena Betancor,&nbsp;Fernando López-Gallego\",\"doi\":\"10.1002/adfm.202470261\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><b>Enzyme Immobilization</b></p><p>In article number 2406097, Fernando López-Gallego and co-workers develop a universal method for encapsulating single gram-negative microbes with polymeric coatings to fabricate synthetic spores that selectively bind His-tagged enzymes. These synthetic spores serve as biocatalytic materials for the one-pot oxidative amination of diols into amino alcohols, facilitated by the cooperative catalysis between intracellular and extracellular enzymes that maintain their performance in consecutive batch cycles.\\n\\n <figure>\\n <div><picture>\\n <source></source></picture><p></p>\\n </div>\\n </figure></p>\",\"PeriodicalId\":112,\"journal\":{\"name\":\"Advanced Functional Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":18.5000,\"publicationDate\":\"2024-11-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adfm.202470261\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Functional Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/adfm.202470261\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Functional Materials","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/adfm.202470261","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

酶固定化在文章编号 2406097 中,Fernando López-Gallego 及其合作者开发了一种通用方法,用聚合物涂层包裹单个革兰氏阴性微生物,从而制造出可选择性结合 His 标记酶的合成孢子。这些合成孢子可作为生物催化材料,用于将二元醇氧化胺化为氨基醇的一锅式反应,细胞内和细胞外酶之间的协同催化作用促进了这种反应,使其在连续的批处理循环中保持性能。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Artificial Spores as Multi-Functional Biocatalysts to Perform Biosynthetic Cascades (Adv. Funct. Mater. 45/2024)

Artificial Spores as Multi-Functional Biocatalysts to Perform Biosynthetic Cascades (Adv. Funct. Mater. 45/2024)

Enzyme Immobilization

In article number 2406097, Fernando López-Gallego and co-workers develop a universal method for encapsulating single gram-negative microbes with polymeric coatings to fabricate synthetic spores that selectively bind His-tagged enzymes. These synthetic spores serve as biocatalytic materials for the one-pot oxidative amination of diols into amino alcohols, facilitated by the cooperative catalysis between intracellular and extracellular enzymes that maintain their performance in consecutive batch cycles.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信