关于 "激子绝缘体 Ta2NiSe5 中隧道尖端诱导的电荷间隙塌缩 "的评论

Dowook Kim, So Young Kim, Jun Sung Kim, Arthur P. Baddorf, An-Ping Li, Tae-Hwan Kim
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引用次数: 0

摘要

在本研究中,我们调查了何其钦等人[Phys. Rev. Res. 3, L032074 (2021)]的估计与最近的角度分辨光发射光谱调查[C. Chen 等人,Phys. Rev. Res. 5, 043089 (2023)]之间的差异,何其钦等人观察到由于扫描隧道显微镜(STM)针尖与样品之间的静电场导致 Ta2NiSe5 中激子间隙的显著塌缩。有人提出,造成这种差异的一个关键因素是 He 等人假设 STM 针尖的功函数是恒定的。这一假设导致对针尖感应电场的低估。使用文献中的样品功函数值,可以得到更可观的电场强度,从而解决了这两种技术在掺杂估计值上的明显冲突。此外,我们的研究结果还强调了 STM 针尖条件的重要性,它可以显著影响针尖功函数,进而影响涉及针尖诱导电场的实验中的掺杂估计。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Comment on “Tunneling-tip-induced collapse of the charge gap in the excitonic insulator Ta2NiSe5”

Comment on “Tunneling-tip-induced collapse of the charge gap in the excitonic insulator Ta2NiSe5”
In this study, we investigate the discrepancy between the estimate of Q. He et al. [Phys. Rev. Res. 3, L032074 (2021)], who observed a remarkable collapse of the exciton gap in Ta2NiSe5 due to the electrostatic field between the scanning tunneling microscope (STM) tip and the sample, and that of a recent angle-resolved photoemission spectroscopy investigation [C. Chen et al., Phys. Rev. Res. 5, 043089 (2023)]. It is proposed that a critical factor contributing to this discrepancy is due to He et al.'s assumption of a constant work function of the STM tip. This assumption led to an underestimation of the tip-induced electric field. Using a literature value for the sample work function, a more substantial electric field strength is obtained, which resolves the apparent conflict between the doping estimates of these two techniques. Furthermore, our findings highlight the importance of the STM tip condition, which can significantly impact the tip work function and, consequently, influence the doping estimation in experiments involving tip-induced electric fields.
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