主动循环波茨模型的时空模式

Hiroshi Noguchi, Jean-Baptiste Fournier
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引用次数: 0

摘要

利用蒙特卡罗模拟和连续统一理论,研究了在方晶格上循环三态波特斯模型的非平衡态动力学。该模型与催化表面上的化学反应和分子跨膜传输有关。根据连续状态之间的翻转能量和相邻位点之间的接触能量,形成了几种特征模式。在循环对称条件下,低翻转能和高翻转能分别形成循环均相和螺旋波。在中间翻转能量机制中,这两种模式在小系统中和/或在低接触能量下暂时共存。在不对称条件下,我们观察到小型双相域表现出类似阿米巴的运动,螺旋波与占主导地位的非循环单态相在时间上共存。在保持其他翻转能量不变的情况下,增加两个连续状态(如状态 0 和状态 1)之间的翻转能量,会诱发第三阶段(状态 2)的形成,这是由于状态 0 域的成核受到抑制。在接触能量不对称的条件下,由于滞后现象,会出现两种不同的模式,这取决于初始状态。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Spatiotemporal patterns in the active cyclic Potts model
The nonequilibrium dynamics of a cycling three state Potts model is studied on a square lattice using Monte Carlo simulations and continuum theory. This model is relevant to chemical reactions on a catalytic surface and to molecular transport across a membrane. Several characteristic modes are formed depending on the flipping energies between successive states and the contact energies between neighboring sites. Under cyclic symmetry conditions, cycling homogeneous phases and spiral waves form at low and high flipping energies, respectively. In the intermediate flipping energy regime, these two modes coexist temporally in small systems and/or at low contact energies. Under asymmetric conditions, we observed small biphasic domains exhibiting amoeba-like locomotion and temporal coexistence of spiral waves and a dominant non-cyclic one-state phase. An increase in the flipping energy between two successive states, say state 0 and state 1, while keeping the other flipping energies constant, induces the formation of the third phase (state 2), owing to the suppression of the nucleation of state 0 domains. Under asymmetric conditions regarding the contact energies, two different modes can appear depending on the initial state, due to a hysteresis phenomenon.
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