非磁性离子辐照下 CrSBr 薄片中铁磁性的消长

Fangchao Long, Yi Li, Yu Cheng, Kseniia Mosina, Ulrich Kentsch, Zdenek Sofer, Slawomir Prucnal, Manfred Helm, Shengqiang Zhou
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引用次数: 0

摘要

通过非磁性离子辐照,探索了 CrSBr 薄片中的磁性相变,揭示了二维(2D)材料中磁性控制的一种新方法。随着辐照通量的增加,在反铁磁性 CrSBr 中观察到了铁磁相的上升和下降。辐照后的 CrSBr 显示出 110 至 84 K 的铁磁临界温度,远高于液态 N2 温度。拉曼光谱显示了声子软化,表明缺陷的形成。这些发现不仅凸显了 CrSBr 在自旋电子学中的潜力,而且还表明离子辐照是调整二维材料磁性能的有效工具,为开发基于空气稳定范德华半导体的自旋电子器件开辟了新途径。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Rise and Fall of the Ferromagnetism in CrSBr Flakes by Non-Magnetic Ion Irradiation

Rise and Fall of the Ferromagnetism in CrSBr Flakes by Non-Magnetic Ion Irradiation

The magnetic phase transition is explored in CrSBr flakes through non-magnetic ion irradiation, revealing a novel method for magnetic control in two-dimensional (2D) materials. The rise and fall of the ferromagnetic phase is observed in antiferromagnetic CrSBr with increasing the irradiation fluence. The irradiated CrSBr shows ferromagnetic critical temperature ranging from 110 to 84 K, well above liquid N2 temperature. Raman spectroscopy reveals phonon softening, suggesting the formation of defects. These findings not only highlight CrSBr's potential in spintronics, but also present ion irradiation as an effective tool for tuning magnetic properties in 2D materials, opening new avenues for the development of spintronic devices based on air-stable van der Waals semiconductors.

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