环形通道中拉长气泡对剪切稀化粘弹性流体的沉积作用与弱弹性机制

Droplet Pub Date : 2024-04-23 DOI:10.1002/dro2.121
SungGyu Chun, Zhengyu Yang, Jie Feng
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引用次数: 0

摘要

流体薄膜沉积在表面涂层、聚合物加工和生物医学设备制造等广泛的工程和生物应用中无处不在。虽然人们已经对牛顿流体中的粘性薄膜沉积进行了广泛研究,但对于经常遇到的非牛顿复杂流体中的沉积动力学,人们仍然无法找到薄膜厚度的预测缩放规律。在此,我们研究了剪切稀化粘弹性流体薄膜在圆形毛细管中平移的长气泡运动中的沉积问题。考虑到具有剪切稀化粘度的弱弹性体系,我们通过系统实验对薄膜厚度进行了定量测量。考虑到有效毛细管数和有效韦森伯格数分别描述了剪切稀化效应和粘弹性效应对薄膜形成的影响,我们进一步利用最近开发的流体动力润滑理论,定量合理地解释了我们的实验观察结果。对于所有测试流体,所获得的缩放定律与实验测量的薄膜厚度相当吻合。我们的工作有可能从根本上推动对封闭几何体中薄膜沉积的理解,并为包含薄膜流和非牛顿流体的过程提供有价值的工程指导。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

Deposition of shear-thinning viscoelastic fluids by an elongated bubble in a circular channel regarding the weakly elastic regime

Deposition of shear-thinning viscoelastic fluids by an elongated bubble in a circular channel regarding the weakly elastic regime

Thin-film deposition of fluids is ubiquitous in a wide range of engineering and biological applications, such as surface coating, polymer processing, and biomedical device fabrication. While the thin viscous film deposition in Newtonian fluids has been extensively investigated, the deposition dynamics in frequently encountered non-Newtonian complex fluids remain elusive, with respect to predictive scaling laws for the film thickness. Here, we investigate the deposition of thin films of shear-thinning viscoelastic fluids by the motion of a long bubble translating in a circular capillary tube. Considering the weakly elastic regime with a shear-thinning viscosity, we provide a quantitative measurement of the film thickness with systematic experiments. We further harness the recently developed hydrodynamic lubrication theory to quantitatively rationalize our experimental observations considering the effective capillary number C a e $Ca_\mathrm{e}$ and the effective Weissenberg number W i e $Wi_\mathrm{e}$ , which describe the shear-thinning and the viscoelastic effects on the film formation, respectively. The obtained scaling law agrees reasonably well with the experimentally measured film thickness for all test fluids. Our work may potentially advance the fundamental understanding of the thin-film deposition in a confined geometry and provide valuable engineering guidance for processes that incorporate thin-film flows and non-Newtonian fluids.

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CiteScore
6.60
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