通过高能电子散射研究氪的广义振子强度和积分截面

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Wan-Lu Ma, Shu-Xing Wang, Zhi-Wei Nie, Jian-Hui Zhu, Jin-Feng Chen, Lin-Fan Zhu
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引用次数: 0

摘要

在入射电子能量为 1500 eV、能量分辨率约为 80 meV 的条件下,测定了氪价壳激发的绝对广义振荡器强度。通过使用稀释目标的相对流技术,排除了压力效应,提高了测量广义振荡器强度的精度。通过将目前的广义振荡器强度与之前的实验和理论结果进行比较,发现在动量传递平方大于 1 a.u. 时并没有达到第一玻恩近似。光学振荡器强度是通过将测量到的广义振荡器强度外推到零平方动量传递得到的,这与之前的电子撞击和光吸收结果进行了交叉检验。借助 BE 缩放法,确定了从激发阈值到 5000 eV 的氪积分截面。目前的振子强度和积分截面补充了氪电子散射的基础数据库,并为理论方法提供了基准。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Generalized oscillator strengths and integral cross sections of krypton studied by high-energy electron scattering

Absolute generalized oscillator strengths of the valence-shell excitations of krypton have been determined with an incident electron energy of 1500 eV and an energy resolution of about 80 meV. By employing the relative flow technique with a dilute target, the pressure effect is excluded and the accuracy of the measured generalized oscillator strengths is improved. By comparing the present generalized oscillator strengths with the previous experimental and theoretical results, it is found that the first Born approximation is not reached at the squared momentum transfer larger than 1 a.u.. The optical oscillator strengths have been obtained by extrapolating the measured generalized oscillator strengths to zero squared momentum transfer, which cross-checks the previous electron impact and photoabsorption results. With the aid of the BE-scaling method, the integral cross sections of krypton have been determined from the excitation threshold to 5000 eV. The present oscillator strengths and integral cross sections supplement the fundamental database of the electron scattering of krypton and provide a benchmark for the theoretical methods.

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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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