{"title":"二维 1T 相氧化铱中的反铁磁性","authors":"Charlie Jindrich;Qi Shao;Antonio Ruotolo","doi":"10.1109/LMAG.2024.3350438","DOIUrl":null,"url":null,"abstract":"Theoretical studies show that metastable phases of nonmagnetic oxides could exhibit magnetic order when synthesized in two-dimensional (2-D) atomic crystals. In this letter, we report experimental evidence of a nontrivial antiferromagnetic behavior in a 2-D, metastable phase of iridium oxide in which iridium forms a triangular lattice. We compare the magnetic behavior of the crystals in the morphology of 2-D nanosheets with that of the same crystals in the morphology of nanoparticles. At low temperatures, the magnetic moment of nanosheets exceeds that of the nanoparticles while coercivity and remanence collapse, suggesting a transition to an antiferromagnetic phase. Morphology at the nanoscale seems to play a significant role in the magnetic behavior of oxide semiconductors.","PeriodicalId":13040,"journal":{"name":"IEEE Magnetics Letters","volume":"15 ","pages":"1-4"},"PeriodicalIF":1.1000,"publicationDate":"2024-01-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Antiferromagnetism in Two-Dimensional, 1T-Phase Iridium Oxide\",\"authors\":\"Charlie Jindrich;Qi Shao;Antonio Ruotolo\",\"doi\":\"10.1109/LMAG.2024.3350438\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Theoretical studies show that metastable phases of nonmagnetic oxides could exhibit magnetic order when synthesized in two-dimensional (2-D) atomic crystals. In this letter, we report experimental evidence of a nontrivial antiferromagnetic behavior in a 2-D, metastable phase of iridium oxide in which iridium forms a triangular lattice. We compare the magnetic behavior of the crystals in the morphology of 2-D nanosheets with that of the same crystals in the morphology of nanoparticles. At low temperatures, the magnetic moment of nanosheets exceeds that of the nanoparticles while coercivity and remanence collapse, suggesting a transition to an antiferromagnetic phase. Morphology at the nanoscale seems to play a significant role in the magnetic behavior of oxide semiconductors.\",\"PeriodicalId\":13040,\"journal\":{\"name\":\"IEEE Magnetics Letters\",\"volume\":\"15 \",\"pages\":\"1-4\"},\"PeriodicalIF\":1.1000,\"publicationDate\":\"2024-01-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"IEEE Magnetics Letters\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://ieeexplore.ieee.org/document/10381849/\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"ENGINEERING, ELECTRICAL & ELECTRONIC\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"IEEE Magnetics Letters","FirstCategoryId":"101","ListUrlMain":"https://ieeexplore.ieee.org/document/10381849/","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
Antiferromagnetism in Two-Dimensional, 1T-Phase Iridium Oxide
Theoretical studies show that metastable phases of nonmagnetic oxides could exhibit magnetic order when synthesized in two-dimensional (2-D) atomic crystals. In this letter, we report experimental evidence of a nontrivial antiferromagnetic behavior in a 2-D, metastable phase of iridium oxide in which iridium forms a triangular lattice. We compare the magnetic behavior of the crystals in the morphology of 2-D nanosheets with that of the same crystals in the morphology of nanoparticles. At low temperatures, the magnetic moment of nanosheets exceeds that of the nanoparticles while coercivity and remanence collapse, suggesting a transition to an antiferromagnetic phase. Morphology at the nanoscale seems to play a significant role in the magnetic behavior of oxide semiconductors.
期刊介绍:
IEEE Magnetics Letters is a peer-reviewed, archival journal covering the physics and engineering of magnetism, magnetic materials, applied magnetics, design and application of magnetic devices, bio-magnetics, magneto-electronics, and spin electronics. IEEE Magnetics Letters publishes short, scholarly articles of substantial current interest.
IEEE Magnetics Letters is a hybrid Open Access (OA) journal. For a fee, authors have the option making their articles freely available to all, including non-subscribers. OA articles are identified as Open Access.