利用石墨烯氧化物砂复合材料 (GOSC) 的吸附作用去除受污染水溶液中的 Pb2+ 离子,实现高效水净化

Q4 Earth and Planetary Sciences
Nidhi Khare, Smarika Lawrence, Amita Chhatri
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引用次数: 0

摘要

铅是一种重金属,会影响人体的所有系统。利用氧化石墨烯涂层砂粒(GOSC)开发了一种去除铅污染的简便方法。在这项研究中,GOSC 是用砂粒和蔗糖溶液在受控加热程序下制备的,与其他吸附剂相比,它具有高效的吸附行为。在 100 ppm 的吸附剂溶液中,只需少量 GOSC(0.09g),GOSC 就能快速去除 Pb+2。在吸附铅离子(Pb2+)之前和之后,使用傅立叶变换红外光谱(FTIR)、X射线衍射(XRD)、扫描电子显微镜(SEM)、电子衍射光(EDX)、电子显微镜(TEM)、电荷耦合(DSC)和 Zeta 电位测量等先进技术对 GOSC 进行了表征。与其他方法相比,吸附法具有更高的去除效率(90% 以上)。研究了各种参数,如时间、pH 值、吸附剂、剂量效应、浓度和温度的影响。结果表明,铅(Pb2+)离子的去除遵循朗缪尔等温线(R2=99%)、二阶动力学(R2=98%)和较高的粒子内扩散(R2=98%)。用少量的 GOSC 就能达到很高的金属离子去除率,这证实 GOSC 是一种优良、有效和经济的吸附剂。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Pb2+ ion removal from contaminated aqueous solution by adsorption onto Graphene Oxide Sand Composite (GOSC) for efficient water purification
Lead is a heavy metal which affects all the systems of human body. An easy method for removal of lead contamination was developed by using graphene oxide coated sand particle (GOSC). In this study, GOSC was prepared using sand particle and sucrose solution under controlled heating program which shows efficient adsorption behavior compared to other adsorbents. GOSC offered very fast removal of Pb+2 with small amount of GOSC (0.09g) in 100 ppm adsorbate solution. Characterization of GOSC was done by using several advanced techniques like FTIR, XRD, SEM, EDX, TEM, DSC, and Zeta Potential measurements before and after adsorption of lead ion (Pb2+). Adsorption shows superiority over other methods because it involves effective and high removal efficiency adsorption (above 90%). Various parameters like the effect of time, pH, adsorbent, dose effect, concentration and temperature were studied. Various adsorption and kinetic models were also investigated using adsorption data and results showed that removal of lead (Pb2+) ion follows Langmuir isotherm (R2 = 99%), second order kinetics (R2 = 98%) and higher intraparticle diffusion (R2= 98%). The high percentage removal of metal ions with little quantity of GOSC confirmed that GOSC is an excellent, effective and economic adsorbent.
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来源期刊
CiteScore
0.50
自引率
0.00%
发文量
195
审稿时长
4-8 weeks
期刊介绍: Information not localized
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