碳酸盐岩层序中封闭性断裂存在下CO2捕集能力的定量评价

A. Fathy, M. Arif, A. Adila, A. Raza, Mohamed Mahmoud
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摘要

矿物捕获被认为是最安全、最可靠的二氧化碳封存技术,注入的二氧化碳可以在地下地层中长期(超过102 - 103年)地质上矿化。然而,与CO2捕集能力预测相关的高复杂性模糊了对CO2矿化的深入理解。本文采用数值模拟的方法,论证了封闭断层存在时碳酸盐矿物学对CO2捕集能力的影响。模拟了三种不同碳酸盐矿物的野外CO2先导地形模型,以描述矿物捕获能力。因此,实际的岩石物理参数、储层特征曲线和其他原位条件被放大以模拟碳酸盐岩地层。然后,对不同成分的储层估算CO2矿化量。此外,通过沉淀/溶解动力学计算,评估了注入压力对CO2矿化的影响。此外,还评价了井位和射孔深度对方解石、白云石和菱铁矿优势储层捕集潜力的影响。圈闭能力计算结果表明,随着注入压力的增加(注底压力至1.5*注底压力),方解石和白云石的圈闭能力单调增加。然而,菱铁矿似乎对注入压力的增加略有不敏感。这种单调趋势是由于随着注入压力的增加,径向位移增强,羽流向上运移受到限制。此外,适当的CO2注入器放置可以显著提高矿物捕获能力,特别是当注入器靠近泄漏侧的断裂面时。该研究对断裂碳酸盐岩层序中CO2矿化潜力的矿物学影响提供了深入的理论认识。这是由于多年来与其他捕获机制相比,对矿物捕获的兴趣微不足道。这是因为矿物捕获需要极长的储存时间才能达到其最大潜力。重要的是,研究结果表明,碳酸盐岩储层中的二氧化碳矿化固定了二氧化碳,从而有助于稳定和长期的永久储存。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Quantitative Assessment of CO2 Mineral Trapping Capacity in Presence of Sealing Fault in Carbonate Sequences: A Numerical Approach
Mineral trapping is believed to be the safest and the most secure CO2 sequestration technique where the injected CO2 could be mineralized in the long-term (exceeding 102 - 103 years) geologically within subsurface formations. Nevertheless, the high complexity associated with CO2 mineral trapping capacity predications obscures the in-depth understanding of CO2 mineralization. In this study, a numerical simulation is adopted to demonstrate the impact of carbonate mineralogy in presence of a sealing fault on CO2 mineral trapping capacity. Field-scale CO2 pilot topographic model for three distinct carbonate minerals is simulated to depict the mineral trapping capacity. Thus, realistic petrophysical parameters, reservoir characteristic curves, and other in-situ conditions are upscaled to mimic carbonate formations. Thereafter, the amount of CO2 mineralized is estimated for compositionally distinct reservoirs. Additionally, the effect of injection pressure on CO2 mineralization is assessed upon precipitation/dissolution kinetics calculations. Moreover, the effects of well placement and perforation depth on mineral trapping potential of calcite, dolomite, and siderite dominant reservoirs are assessed. The mineral trapping capacities computed show that increasing injection pressure (base injection pressure to 1.5*base injection pressure) monotonically increased the mineral trapping capacities for calcite and dolomite. However, siderite seems slightly insensitive to the injection pressure increase. This monotonic trend is attributed to enhanced radial displacement and restricted plume migration upward as the injection pressure increases. Moreover, proper CO2 injector placement showed significant enhancement in mineral trapping capacity especially if the injector is near to the fault plane on the leaking side. This study provides in-depth theoretical understanding of the mineralogy effect on CO2 mineralization potential in faulty carbonate sequences. This is driven by the insignificance interest mineral trapping has gained over the years compared to other trapping mechanisms. This is because of the extremely long storage duration needed for mineral trapping to reach its maximum potential. Importantly, the results suggest that CO2 mineralization within carbonate reservoirs immobilize CO2 – thus assisting in stable and long-term permanent storage.
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