纳米结构的光-热耗散:从超快光调制到蒸汽产生

A. Alabastri
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引用次数: 0

摘要

纳米结构在与辐射相互作用时储存能量的方式不同,这取决于所考虑的时间尺度、系统大小和相互作用的组件。适当设计的纳米结构表面限制了电磁能量,使其成为高能电子和受限场、远场散射、热或热辐射。本次演讲将展示金属纳米结构中的空间非均匀电磁吸收如何导致空间依赖的非平衡热载流子群,其< 1 ps的热化可以用于超快全光偏振调制。最终,热量通过一个较慢的电子-声子散射过程产生。我将展示超薄(~250nm)等离子体超表面如何吸收~90%的太阳光谱,导致~GW/m3的耗散功率被利用,例如,用于蒸汽产生,与灭菌或海水淡化应用相关。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
Light-to-heat dissipation in nanoscale structures: from ultrafast optical modulation to steam generation
Nanostructures store energy differently upon interaction with radiation, depending on the considered time scale, system size, and interacting components. Properly designed nanostructured surfaces confine electromagnetic energy, making it available as high energy electrons and confined fields, far-field scattering, heat or thermal radiation. This talk will show how the spatially inhomogeneous electromagnetic absorption in metallic nanostructures leads to a space-dependent out-of-equilibrium hot carrier population, whose < 1 ps thermalization can be exploited for ultrafast all-optical polarization modulation. Eventually, heat is generated through a slower electron-phonon scattering process. I will show how ultrathin (~250nm) plasmonic metasurfaces can absorb ~90% of the solar spectrum, leading to ~GW/m3 of dissipated power exploited, for example, for steam generation, relevant for sterilization or water desalination applications.
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