Ultrafast x-ray imaging of pulsed plasmas in water

Abstract

Pulsed plasmas in liquids exhibit complex interaction between three phases of matter (liquids, gas, plasmas) and are currently used in a wide range of applications across several fields, however significant knowledge gaps in our understanding of plasma initiation in liquids hinder additional application and control; this area of research currently lacks a comprehensive predictive model. To aid progress in this area experimentally, here we present the first-known ultrafast (50 ps) X-ray images of pulsed plasma initiation processes in water (+25 kV, 10 ns, 5 mJ), courtesy of the X-ray imaging techniques available at Argonne National Laboratory's Advanced Photon Source (APS), with supporting nanosecond optical imaging and a computational X-ray diffraction model. These results clearly resolve narrow (~10 micron) low-density plasma channels during initiation timescales typically obscured by optical emission (<100 ns), a well-known and difficult problem to plasma experiments without access to state-of-the-art X-ray sources such as the APS synchrotron. Images presented in this work speak to several of the prevailing plasma initiation hypotheses, supporting electrostriction and bubble deformation as dominant initiation phenomena. We also demonstrate the plasma setup used in this work as a cheap ($<$US\$100k), compact, and repeatable benchmark imaging target (29.1 km/s, 1 TW/cm$^2$) useful for the development of next-generation ultrafast imaging of high-energy-density physics (HEDP), as well as easier integration of HEDP research into synchrotron-enabled facilities.