Atomic diffusion in liquid Ni, NiP, PdNiP, and PdNiCuP alloys

IF 3.5 2区 物理与天体物理 Q2 PHYSICS, APPLIED
S. M. Chathoth, A. Meyer, M. Koza, F. Jurányi
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引用次数: 72

Abstract

We investigated the self-diffusion of Ni in liquid Ni, Ni80P20, Pd40Ni40P20, and Pd43Ni10Cu27P20 at temperatures up to 1795K with incoherent, quasielastic neutron scattering. Values of measured self-diffusion coefficients vary over the accessible temperature ranges as a function of composition only within 10%. Although mixing has a drastic effect on the liquidus temperature and the undercooling capabilities, a relation between these properties and the atomic diffusion in the liquid is not observed. Apparently, diffusive motion is governed by the packing fraction of the atoms, that is very similar in these dense liquids.
Ni、NiP、PdNiP和PdNiCuP合金液体中的原子扩散
利用非相干准弹性中子散射研究了Ni在液态Ni、Ni80P20、Pd40Ni40P20和Pd43Ni10Cu27P20中在1795K温度下的自扩散。测量的自扩散系数值在可达到的温度范围内作为成分的函数变化仅在10%以内。虽然混合对液体温度和过冷能力有很大的影响,但这些性质与液体中的原子扩散之间的关系没有观察到。显然,扩散运动是由原子的堆积率决定的,这在这些致密液体中非常相似。
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来源期刊
Applied Physics Letters
Applied Physics Letters 物理-物理:应用
CiteScore
6.40
自引率
10.00%
发文量
1821
审稿时长
1.6 months
期刊介绍: Applied Physics Letters (APL) features concise, up-to-date reports on significant new findings in applied physics. Emphasizing rapid dissemination of key data and new physical insights, APL offers prompt publication of new experimental and theoretical papers reporting applications of physics phenomena to all branches of science, engineering, and modern technology. In addition to regular articles, the journal also publishes invited Fast Track, Perspectives, and in-depth Editorials which report on cutting-edge areas in applied physics. APL Perspectives are forward-looking invited letters which highlight recent developments or discoveries. Emphasis is placed on very recent developments, potentially disruptive technologies, open questions and possible solutions. They also include a mini-roadmap detailing where the community should direct efforts in order for the phenomena to be viable for application and the challenges associated with meeting that performance threshold. Perspectives are characterized by personal viewpoints and opinions of recognized experts in the field. Fast Track articles are invited original research articles that report results that are particularly novel and important or provide a significant advancement in an emerging field. Because of the urgency and scientific importance of the work, the peer review process is accelerated. If, during the review process, it becomes apparent that the paper does not meet the Fast Track criterion, it is returned to a normal track.
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